Facile fabrication of fibrous Bi4Ti3O12/Bi2S3/MoS2with enhanced photocatalytic activities towards pollutant degradation under visible light irradiation

被引:8
|
作者
Liu, Jun [1 ]
Hui, Qian [1 ]
Chang, Meng-Jie [1 ]
Cui, Wen-Na [1 ]
Xi, Tong [1 ]
Wang, Lin-Da [1 ]
Sun, Meng [1 ]
Yuan, Bin [1 ]
Ni, Fu-Rong [1 ]
机构
[1] Xian Univ Sci & Technol, Dept Mat Sci & Engn, Xian 710054, Peoples R China
基金
中国国家自然科学基金;
关键词
EXPOSED; 001; FACETS; CONTROLLABLE SYNTHESIS; BI4TI3O12; NANOSHEETS; OXYGEN-VACANCY; HETEROSTRUCTURE; HETEROJUNCTION; CONSTRUCTION; NANOFIBERS; TIO2; NANOCOMPOSITES;
D O I
10.1007/s10854-020-04324-4
中图分类号
TM [电工技术]; TN [电子技术、通信技术];
学科分类号
0808 ; 0809 ;
摘要
Herein, novel fibrous Bi4Ti3O12/Bi2S3/MoS(2)is constructed by a simple one-step methodology for photocatalytic degradation of RhB dyes. Bi4Ti3O12/Bi2S3/MoS(2)hybrid fibers were facilely prepared by direct hydrothermal growth of MoS(2)nanosheets on electrospun Bi(4)Ti(3)O(12)nanofiber surface, during which rod-like Bi(2)S(3)was formed by in-situ ion exchange reaction between BTO and S source. The MoS(2)nanosheets with several-layer thickness uniformly are coated both on the BTO and Bi(2)S(3)surface. Remarkable enhancement of visible light absorption and photo-generated charge separation in Bi4Ti3O12/Bi2S3/MoS(2)are achieved compared with the bare BTO nanofibers. By changing the weight ratio of Mo/S and the precursor dosage of MoS2, the optimized BM-150/250 sample presents 2.3 and 4.1 times higher of the photodegradation efficiency and apparent reaction rate constant, respectively, than that of pure BTO fibers after 120-min irradiation under visible light. The system pays an efficient pathway to establish ternary composite fibers providing high photocatalytic activity for other electrospun Bi-contained nanofibers.
引用
收藏
页码:17688 / 17702
页数:15
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