Generation of narrowband pulses from chirped broadband pulse frequency mixing

被引:14
作者
Courtney, Trevor L. [1 ]
Mecker, Nils Torge [2 ]
Patterson, Brian D. [1 ]
Linne, Mark [2 ]
Kliewer, Christopher J. [1 ]
机构
[1] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA
[2] Univ Edinburgh, Sch Engn, Edinburgh EH8 3JL, Midlothian, Scotland
基金
英国工程与自然科学研究理事会;
关键词
STOKES-RAMAN SCATTERING; EFFICIENT GENERATION; MIDINFRARED PULSES; PICOSECOND PULSES; MU-M; SPECTROSCOPY;
D O I
10.1364/OL.44.000835
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We extend an approach based upon sum-frequency generation of oppositely chirped pulses to narrow the bandwidths of broadband femtosecond pulses. We efficiently generate near-transform-limited pulses with durations of several picoseconds, while reducing the pulse bandwidth by a factor of 120, which is more than twice the reduction reported in previous literature. Such extreme bandwidth narrowing of a broadband pulse enhances the effects of dispersion nonlinearities. Precise chirp control enables us to characterize the efficacy of frequency mixing broadband pulses with nonlinear temporal chirps. We demonstrate the use of these narrowband pulses as probes in coherent anti-Stokes Raman spectroscopy. (C) 2019 Optical Society of America
引用
收藏
页码:835 / 838
页数:4
相关论文
共 22 条
[1]   Communication: Simplified two-beam rotational CARS signal generation demonstrated in 1D [J].
Bohlin, Alexis ;
Patterson, Brian D. ;
Kliewer, Christopher J. .
JOURNAL OF CHEMICAL PHYSICS, 2013, 138 (08)
[2]   Narrowband carrier-envelope phase stable mid-infrared pulses at wavelengths beyond 10 μm by chirped-pulse difference frequency generation [J].
Cartella, A. ;
Nova, T. F. ;
Oriana, A. ;
Cerullo, G. ;
Foerst, M. ;
Manzoni, C. ;
Cavalleri, A. .
OPTICS LETTERS, 2017, 42 (04) :663-666
[3]   Hybrid fs/ps rotational CARS temperature and oxygen measurements in the product gases of canonical flat flames [J].
Kearney, Sean P. .
COMBUSTION AND FLAME, 2015, 162 (05) :1748-1758
[4]   Bandwidth optimization of femtosecond pure-rotational coherent anti-Stokes Raman scattering by pump/Stokes spectral focusing [J].
Kearney, Sean P. .
APPLIED OPTICS, 2014, 53 (28) :6579-6585
[5]   Hybrid femtosecond/picosecond rotational coherent anti-Stokes Raman scattering at flame temperatures using a second-harmonic bandwidth-compressed probe [J].
Kearney, Sean P. ;
Scoglietti, Daniel J. .
OPTICS LETTERS, 2013, 38 (06) :833-835
[6]   Generation of narrowband subpicosecond mid-infrared pulses via difference frequency mixing of chirped near-infrared pulses [J].
Koller, Florian O. ;
Haiser, Karin ;
Huber, Markus ;
Schrader, Tobias E. ;
Regner, Nadja ;
Schreier, Wolfgang J. ;
Zinth, Wolfgang .
OPTICS LETTERS, 2007, 32 (22) :3339-3341
[7]   An efficient setup for femtosecond stimulated Raman spectroscopy [J].
Kovalenko, S. A. ;
Dobryakov, A. L. ;
Ernsting, N. P. .
REVIEW OF SCIENTIFIC INSTRUMENTS, 2011, 82 (06)
[8]   A femtosecond stimulated raman spectrograph for the near ultraviolet [J].
Laimgruber, S. ;
Schachenmayr, H. ;
Schmidt, B. ;
Zinth, W. ;
Gilch, P. .
APPLIED PHYSICS B-LASERS AND OPTICS, 2006, 85 (04) :557-564
[9]   Femtosecond broadband stimulated Raman spectroscopy: Apparatus and methods [J].
McCamant, DW ;
Kukura, P ;
Yoon, S ;
Mathies, RA .
REVIEW OF SCIENTIFIC INSTRUMENTS, 2004, 75 (11) :4971-4980
[10]   Femtosecond time-resolved stimulated Raman spectroscopy:: Application to the ultrafast internal conversion in β-carotene [J].
McCamant, DW ;
Kukura, P ;
Mathies, RA .
JOURNAL OF PHYSICAL CHEMISTRY A, 2003, 107 (40) :8208-8214