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Solution-phase epitaxial growth of noble metal nanostructures on dispersible single-layer molybdenum disulfide nanosheets
被引:757
作者:

Huang, Xiao
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Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore

Zeng, Zhiyuan
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Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore

Bao, Shuyu
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Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore

Wang, Mengfei
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Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore

Qi, Xiaoying
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Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore

Fan, Zhanxi
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Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore

Zhang, Hua
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Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore
机构:
[1] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore
基金:
新加坡国家研究基金会;
关键词:
GRAPHENE;
NANOCRYSTALS;
NANOPARTICLES;
AU;
REDUCTION;
PD;
SEMICONDUCTOR;
NANOPRISMS;
OXIDATION;
NANORODS;
D O I:
10.1038/ncomms2472
中图分类号:
O [数理科学和化学];
P [天文学、地球科学];
Q [生物科学];
N [自然科学总论];
学科分类号:
07 ;
0710 ;
09 ;
摘要:
Compared with the conventional deposition techniques used for the epitaxial growth of metallic structures on a bulk substrate, wet-chemical synthesis based on the dispersible template offers several advantages, including relatively low cost, high throughput, and the capability to prepare metal nanostructures with controllable size and morphology. Here we demonstrate that the solution-processable two-dimensional MoS2 nanosheet can be used to direct the epitaxial growth of Pd, Pt and Ag nanostructures at ambient conditions. These nanostructures show the major (111) and (101) orientations on the MoS2(001) surface. Importantly, the Pt-MoS2 hybrid nanomaterials exhibit much higher electrocatalytic activity towards the hydrogen evolution reaction compared with the commercial Pt catalysts with the same Pt loading. We believe that nanosheet-templated epitaxial growth of nanostructures via wet-chemical reaction is a promising strategy towards the facile and high-yield production of novel functional materials.
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