Natural Gas to Fuels and Chemicals: Improved Methane Aromatization in an Oxygen-Permeable Membrane Reactor

被引：95

作者：

Cao, Zhengwen ^{[1
]}

Jiang, Heqing ^{[2
]}

Luo, Huixia ^{[1
,3
]}

Baumann, Stefan ^{[4
]}

Meulenberg, Wilhelm A. ^{[4
]}

Assmann, Jens ^{[5
]}

Mleczko, Leslaw ^{[5
]}

Liu, Yi ^{[1
]}

Caro, Juergen ^{[1
]}

机构：

[1] Leibniz Univ Hannover, Inst Phys Chem & Electrochem, D-30167 Hannover, Germany

[2] Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Key Lab Biobased Mat, Qingdao 266101, Peoples R China

[3] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA

[4] Forschungszentrum Julich GmbH, Inst Energy & Climate Res, D-52425 Julich, Germany

[5] Bayer Technol Serv GmbH, BTS TD UP Chem Catalysis, D-51368 Leverkusen, Germany

来源：

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION | 2013年 / 52卷 / 51期

关键词：

aromatic compounds; dehydroaromatization; membrane reactors; methane; oxygen-permeable membranes; NONOXIDATIVE ACTIVATION; CATALYTIC PERFORMANCE; HYDROGEN-PRODUCTION; WATER DISSOCIATION; CONVERSION; MO/HZSM-5; PEROVSKITE; DEHYDROAROMATIZATION; DEHYDROGENATION; REDUCTION;

D O I：

10.1002/anie.201307935

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Adding value with membranes: Improved methane aromatization was achieved by using an oxygen-permeable membrane. The resulting membrane reactor shows a superior methane conversion and a higher resistance towards catalyst deactivation. Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

引用

页码：13794 / 13797

页数：4

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