Occurrence, distribution, and bioaccumulation of antibiotics in coastal environment of Dalian, China

被引:170
作者
Na, Guangshui [1 ,2 ]
Fang, Xiaodan [1 ]
Cai, Yaqi [2 ]
Ge, Linke [1 ]
Zong, Humin [1 ]
Yuan, Xiutang [1 ]
Yao, Ziwei [1 ]
Zhang, Zhifeng [1 ]
机构
[1] Natl Marine Environm Monitoring Ctr, Key Lab Ecol Environm Coastal Areas SOA, Dalian, Peoples R China
[2] Chinese Acad Sci, Ecoenvironm Sci Res Ctr, Beijing, Peoples R China
基金
中国国家自然科学基金;
关键词
Antibiotics; Occurrence; Seawater; Sediments; Aquatic organisms; Dalian; TANDEM MASS-SPECTROMETRY; RIVER DISCHARGE; SEDIMENTS; IMPACTS; WATERS;
D O I
10.1016/j.marpolbul.2012.12.028
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Seawater, sediment, and aquatic organism samples were collected from 20 sampling sites in coastal environment of Dalian in August, 2011. The occurrence, distribution, and bioaccumulation of 20 antibiotics categorizing into three groups, including 14 sulfonamides (SAs), two chloramphenicols (CAPS) and four tetracyclines (TCs), were investigated. The results suggested that tetracyclines were the predominant antibiotics in the seawater (range: 2.11-9.23 ng L-1), while sulfonamides were the dominant antibiotics in both sediments (range: 1.42-71.32 mu g kg(-1)) and aquatic organisms (range: 2.18-63.87 mu g kg(-1)). The sorption coefficient K-d,K-s values revealed that sulfameter, sulfadiazine, sulfamethoxypyridazine, sulfamonomethoxine, chloramphenicol, and doxycycline presented higher sorption capacities than the other antibiotics. The average BAFs suggested that sulfamethazine, sulfamethiazole, sulfamonomethoxine, and doxycycline were potentially bioaccumulative, while sulfadiazine, sulfameter, sulfamethoxypyridazine, and chloramphenicol were bioaccumulative. (C) 2013 Published by Elsevier Ltd.
引用
收藏
页码:233 / 237
页数:5
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