NOx SCALING OF SYNGAS H2/CO TURBULENT NON-PREMIXED JET FLAMES

被引:23
作者
Hwang, Jeongjae [1 ]
Sohn, Kitae [1 ]
Bouvet, Nicolas [1 ]
Yoon, Youngbin [1 ]
机构
[1] Seoul Natl Univ, Sch Mech & Aerosp Engn, Seoul, South Korea
关键词
EINOx; Hydrogen flame; Non-premixed jet flame; NOx scaling; Syngas; DIFFUSION FLAMES; HYDROGEN JET; COMBUSTION; MIXTURES; IGNITION; GAS; TEMPERATURE; EMISSIONS; KINETICS; DILUTION;
D O I
10.1080/00102202.2013.831847
中图分类号
O414.1 [热力学];
学科分类号
摘要
NOx emission characteristics and EINOx scaling of hydrogen and H-2/CO syngas non-premixed jet flames under turbulent condition are investigated. Flame length and NOx concentration were measured simultaneously for four different syngas compositions (100/0, 75/25, 50/50, and 25/75 H-2/CO% vol.) and three different fuel nozzle diameters (2.5, 3.0, and 3.5mm). The jet flames were in the buoyancy-momentum transition regime. NOx emission is reduced with increased Reynolds number and increased CO content in the syngas fuel, which result from a decreased flame residence time. The previous EINOx scaling correlation, which is based on flame residence time (flame volume divided by volume flow rate of fuel), does not apply to a hydrogen jet flame in the buoyancy-momentum transition region. The previous scaling applies only to momentum-dominated jet flames. A modified scaling based on a simplified flame residence time (flame length divided by fuel jet velocity) considered the buoyancy effect as proposed. This scaling aligns the 1/2-power with the jet flame in both momentum-dominated and transition regions. The modified scaling also satisfies the 1/2 slope with H-2/CO syngas jet flames. Furthermore, the proposed modified scaling adopts the nitrogen amount as a reference, instead of the fuel amount. Finally, the modified scaling collapses the all syngas compositions into a single line.
引用
收藏
页码:1715 / 1734
页数:20
相关论文
共 35 条
[1]   Experimental studies of the fundamental flame speeds of syngas (H2/CO)/air mixtures [J].
Bouvet, Nicolas ;
Chauveau, Christian ;
Goekalp, Iskender ;
Halter, Fabien .
PROCEEDINGS OF THE COMBUSTION INSTITUTE, 2011, 33 :913-920
[2]   Syngas combustion kinetics and applications [J].
Chaos, Marcos ;
Dryer, Frederick L. .
COMBUSTION SCIENCE AND TECHNOLOGY, 2008, 180 (06) :1053-1096
[3]   PDF MODELING AND ANALYSIS OF THERMAL NO FORMATION IN TURBULENT NONPREMIXED HYDROGEN AIR-JET FLAMES [J].
CHEN, JY ;
KOLLMANN, W .
COMBUSTION AND FLAME, 1992, 88 (3-4) :397-412
[4]  
Chen R. -H., 1990, 23 S INT COMBUSTION, P281
[5]   Turbulent flame speed for syngas at gas turbine relevant conditions [J].
Daniele, S. ;
Jansohn, P. ;
Mantzaras, J. ;
Boulouchos, K. .
PROCEEDINGS OF THE COMBUSTION INSTITUTE, 2011, 33 :2937-2944
[6]  
Daniele S., 2008, GT200850265 ASME
[7]   Laminar flame speeds of moist syngas mixtures [J].
Das, Apurba K. ;
Kumar, Kamal ;
Sung, Chih-Jen .
COMBUSTION AND FLAME, 2011, 158 (02) :345-353
[8]   An optimized kinetic model of H2/CO combustion [J].
Davis, SG ;
Joshi, AV ;
Wang, H ;
Egolfopoulos, F .
PROCEEDINGS OF THE COMBUSTION INSTITUTE, 2005, 30 (01) :1283-1292
[9]   TRANSITION FROM MOMENTUM TO BUOYANCY-CONTROLLED TURBULENT JET DIFFUSION FLAMES AND FLAME HEIGHT RELATIONSHIPS [J].
DELICHATSIOS, MA .
COMBUSTION AND FLAME, 1993, 92 (04) :349-364
[10]   SUPEREQUILIBRIUM AND THERMAL NITRIC-OXIDE FORMATION IN TURBULENT-DIFFUSION FLAMES [J].
DRAKE, MC ;
CORREA, SM ;
PITZ, RW ;
SHYY, W ;
FENIMORE, CP .
COMBUSTION AND FLAME, 1987, 69 (03) :347-365