Syngas Production from Ethanol Dry Reforming over Cu/Ce0.8Zr0.2O2 Catalyst

被引:20
作者
Cao, Dong [1 ]
Cai, Weijie [1 ,3 ]
Li, Yi [2 ]
Li, Congming [3 ]
Yu, Hao [4 ]
Zhang, Shaoyin [1 ]
Qu, Fengzuo [1 ]
机构
[1] Dalian Polytech Univ, Fac Light Ind & Chem Engn, Dalian 116023, Peoples R China
[2] Jilin Univ, Coll Chem, State Key Lab Inorgan Synth & Preparat Chem, Changchun 130012, Jilin, Peoples R China
[3] Taiyuan Univ Technol, State Key Lab Breeding Base Coal Sci & Technol, Taiyuan 030024, Shanxi, Peoples R China
[4] Shandong Univ Sci & Technol, Coll Chem & Environm Engn, Qingdao 266590, Peoples R China
关键词
Cu/Ce0.8Zr0.2O2; Ethanol dry reforming; Syngas; Hydrogen; CO OXIDATION ACTIVITY; HYDROGEN-PRODUCTION; LOW-TEMPERATURE; MIXED OXIDES; CE; CU; ZR; METHANE; CERIA; IMPREGNATION;
D O I
10.1007/s10562-017-2216-0
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
A Cu/Ce0.8Zr0.2O2 catalyst was synthesized by facile co-precipitation method and deeply studied for syngas production from carbon dioxide reforming of ethanol at various temperature and reactant ratios. The investigated catalyst showed promising activity and excellent stability along 90 h test, which was assigned to the strong synergistic metal-support interaction and high redox capacity as revealed by different characterization technique including X-ray diffraction (XRD), Raman, Oxygen storage capacity (OSC) and Temperature programmed reduction (H-2-TPR) etc. [GRAPHICS]
引用
收藏
页码:2929 / 2939
页数:11
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