Interfacial Control of Magnetic Properties at LaMnO3/LaNiO3 Interfaces

被引:96
作者
Gibert, M. [1 ]
Viret, M. [1 ,2 ]
Torres-Pardo, A. [3 ]
Piamonteze, C. [4 ]
Zubko, P. [1 ]
Jaouen, N. [5 ]
Tonnerre, J. -M. [6 ]
Mougin, A. [3 ]
Fowlie, J. [1 ]
Catalano, S. [1 ]
Gloter, A. [3 ]
Stephan, O. [3 ]
Triscone, J. -M. [1 ]
机构
[1] Univ Geneva, Dept Phys Matiere Quant, Geneva, Switzerland
[2] CEA Saclay, CNRS, URA 2464, Serv Phys Etat Condense, F-91191 Gif Sur Yvette, France
[3] Univ Paris 11, Phys Solides Lab, CNRS UMR 8502, F-91405 Orsay, France
[4] Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland
[5] Synchrotron SOLEIL, F-91192 Gif Sur Yvette, France
[6] CNRS, Inst Neel, F-38042 Grenoble, France
基金
瑞士国家科学基金会; 欧洲研究理事会;
关键词
Interface engineering; manganites; nickelates; magnetism; RAY ABSORPTION-SPECTROSCOPY; METAL-INSULATOR-TRANSITION; OXIDE HETEROSTRUCTURES; ELECTRONIC-PROPERTIES; NEUTRON-DIFFRACTION; LOW-TEMPERATURE; ATOMIC-SCALE; SUPERLATTICES; FILMS; FERROMAGNETISM;
D O I
10.1021/acs.nanolett.5b02720
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The functional properties of oxide heterostructures ultimately rely on how the electronic and structural mismatches occurring at interfaces are accommodated by the chosen materials combination. We discuss here LaMnO3/LaNiO3 heterostructures, which display an intrinsic interface structural asymmetry depending on the growth sequence. Using a variety of synchrotron-based techniques, we show that the degree of intermixing at the monolayer scale allows interface-driven properties such as charge transfer and the induced magnetic moment in the nickelate layer to be controlled. Further, our results demonstrate that the magnetic state of strained LaMnO3 thin films dramatically depends on interface reconstructions.
引用
收藏
页码:7355 / 7361
页数:7
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