Measurement of the 230U half-life

被引：15

作者：

Pomme, S. ^{[1
]}

Altzitzoglou, T. ^{[1
]}

Van Ammel, R. ^{[1
]}

Suliman, G. ^{[1
]}

Marouli, M. ^{[1
]}

Jobbagy, V. ^{[1
]}

Paepen, J. ^{[1
]}

Stroh, H. ^{[1
]}

Apostolidis, C. ^{[2
]}

Abbas, K. ^{[3
]}

Morgenstern, A. ^{[2
]}

机构：

[1] European Commiss, Joint Res Ctr, Inst Reference Mat & Measurements, B-2440 Geel, Belgium

[2] European Commiss, Joint Res Ctr, Inst Transuranium Elements, D-76125 Karlsruhe, Germany

[3] European Commiss, Joint Res Ctr, Inst Hlth & Consumer Protect, I-21020 Ispra, VA, Italy

来源：

APPLIED RADIATION AND ISOTOPES | 2012年 / 70卷 / 09期

关键词：

Half-life; U-230; Radionuclide metrology; Nuclear data; Radiotherapy; TARGETED ALPHA THERAPY; PRIMARY STANDARDIZATION;

D O I：

10.1016/j.apradiso.2012.02.053

中图分类号：

O61 [无机化学];

学科分类号：

070301 ; 081704 ;

摘要：

The U-230 half-life was determined by measuring the decay curve of U-230 sources by various nuclear detection techniques: alpha-particle counting at a defined small solid angle; 4 pi alpha+beta counting with a windowless CsI sandwich spectrometer, a liquid scintillation counter and a pressurised proportional counter; gamma-ray spectrometry with a HPGe detector and nearly-2 pi alpha-particle counting with an ion-implanted silicon detector. Depending on the technique, the decay was followed for 100-200 d, which is 5-10 times the U-230 half-life. The measurement results of the various techniques were in good mutual agreement. The mean value, T-1/2(U-230)=20.23 (2) d, is lower than the literature value which is based on one measurement in 1948 and resulted in a half-life value of 20.8 d without statement of uncertainty. A correction for the ingrowth of the long-lived Pb-210 and its daughter products may have been overlooked in the past. (C) 2012 Elsevier Ltd. All rights reserved.

引用

页码：1900 / 1906

页数：7

共 21 条

[1] Nuclear data sheets for A = 226 [J].

Akovali, Y.A. .

Nuclear Data Sheets, 1996, 77 (02) :433-470

[2]

Chiste V., 2008, MONOGRAPHIE BUREAU I, V4, P51

[3] ABSOLUTE ACTIVITY MEASUREMENTS WITH THE WINDOWLESS 4-PI-CSI(TL)-SANDWICH SPECTROMETER [J].

DENECKE, B .

NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT, 1994, 339 (1-2) :92-98

[4]

MANN WB, 1988, APPL RADIAT ISOTOPES, V39, P717

[5] High-resolution alpha-particle spectrometry of the 230U decay series [J].

Marouli, M. ;

Pomme, S. ;

Paepen, J. ;

Van Ammel, R. ;

Jobbagy, V. ;

Dirican, A. ;

Suliman, G. ;

Stroh, H. ;

Apostolidis, C. ;

Abbas, K. ;

Morgenstern, A. .

APPLIED RADIATION AND ISOTOPES, 2012, 70 (09) :2270-2274

[6] Cross sections of the reaction 231Pa(d,3n)230U for the production of 230U/226Th for targeted α therapy [J].

Morgenstern, A. ;

Lebeda, O. ;

Stursa, J. ;

Capote, R. ;

Sin, M. ;

Bruchertseifer, F. ;

Zielinska, B. ;

Apostolidis, C. .

PHYSICAL REVIEW C, 2009, 80 (05)

[7]

Morgenstern A., 2006, Patent, Patent No. [2006003123, WO 2006/003123]

[8] Production of 230U/226Th for Targeted Alpha Therapy via Proton Irradiation of 231Pa [J].

Morgenstern, Alfred ;

Lebeda, Ondrej ;

Stursa, Jan ;

Bruchertseifer, Frank ;

Capote, Roberto ;

McGinley, John ;

Rasmussen, Gert ;

Sin, Mihaela ;

Zielinska, Barbara ;

Apostolidis, Christos .

ANALYTICAL CHEMISTRY, 2008, 80 (22) :8763-8770

[9] Cross-sections of the reaction 232Th(p,3n)230Pa for reaction of 230U production for targeted alpha therapy [J].

Morgenstern, Alfred ;

Apostolidis, Christos ;

Bruchertseifer, Frank ;

Capote, Roberto ;

Gouder, Thomas ;

Simonelli, Federica ;

Sin, Mihaela ;

Abbas, Kamel .

APPLIED RADIATION AND ISOTOPES, 2008, 66 (10) :1275-1280

[10] Targeted Alpha Therapy with Bi-213 [J].

Morgenstern, Alfred ;

Bruchertseifer, Frank ;

Apostolidis, Christos .

CURRENT RADIOPHARMACEUTICALS, 2011, 4 (04) :295-305

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