Gas-liquid mass transfer coefficient of methane in bubble column reactor

被引:9
作者
Lee, Jaewon [1 ]
Yasin, Muhammad [2 ]
Park, Shinyoung [2 ]
Chang, In Seop [2 ]
Ha, Kyoung-Su [1 ]
Lee, Eun Yeol [3 ]
Lee, Jinwon [1 ]
Kim, Choongik [1 ]
机构
[1] Sogang Univ, Dept Chem & Biomol Engn, 1 Shinsoo Dong, Seoul 121742, South Korea
[2] GIST, Sch Environm Sci & Engn, Gwangju 500712, South Korea
[3] Kyung Hee Univ, Dept Chem Engn, Gyeonggi Do 446701, South Korea
关键词
Methane; Mass Transfer Coefficient; Bubble Column Reactor; Shale Gas; SOLUBILITY; SOIL;
D O I
10.1007/s11814-014-0341-7
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Biological conversion of methane gas has been attracting considerable recent interest. However, methanotropic bioreactor is limited by low solubility of methane gas in aqueous solution. Although a large mass transfer coefficient of methane in water could possibly overcome this limitation, no dissolved methane probe in aqueous environment is commercially available. We have developed a reactor enabling the measurement of aqueous phase methane concentration and mass transfer coefficient (k(L)a). The feasibility of the new reactor was demonstrated by measuring k(L)a values as a function of spinning rate of impeller and flow rate of methane gas. Especially, at spinning rate of 300 rpm and flow rate of 3.0 L/min, a large k(L)a value of 102.9 h (1) was obtained.
引用
收藏
页码:1060 / 1063
页数:4
相关论文
共 25 条
[1]   GAS HOLDUP AND VOLUMETRIC MASS-TRANSFER COEFFICIENT IN BUBBLE COLUMNS - EFFECTS OF LIQUID PROPERTIES [J].
AKITA, K ;
YOSHIDA, F .
INDUSTRIAL & ENGINEERING CHEMISTRY PROCESS DESIGN AND DEVELOPMENT, 1973, 12 (01) :76-80
[2]   Gas-liquid mass transfer in dual impeller bioreactor [J].
Arjunwadkar, SJ ;
Sarvanan, K ;
Kulkarni, PR ;
Pandit, AB .
BIOCHEMICAL ENGINEERING JOURNAL, 1998, 1 (02) :99-106
[3]   THE PREDICTION OF METHANE SOLUBILITY IN NATURAL-WATERS TO HIGH IONIC-STRENGTH FROM O-DEGREES-C TO 250-DEGREES-C AND FROM 0 TO 1600 BAR [J].
DUAN, ZH ;
MOLLER, N ;
GREENBERG, J ;
WEARE, JH .
GEOCHIMICA ET COSMOCHIMICA ACTA, 1992, 56 (04) :1451-1460
[4]   A thermodynamic model for calculating methane solubility, density and gas phase composition of methane-bearing aqueous fluids from 273 to 523 K and from 1 to 2000 bar [J].
Duan, Zhenhao ;
Mao, Shide .
GEOCHIMICA ET COSMOCHIMICA ACTA, 2006, 70 (13) :3369-3386
[5]   Requirements for the development of a bioeconomy for chemicals [J].
Dubois, Jean-Luc .
CURRENT OPINION IN ENVIRONMENTAL SUSTAINABILITY, 2011, 3 (1-2) :11-14
[6]   Mass transfer correlations for multiple-impeller gas-liquid contactors.: Analysis of the effect of axial dispersion in gas and liquid phases on "local" kLa values measured by the dynamic pressure method in individual stages of the vessel [J].
Fujasova, M. ;
Linek, V. ;
Moucha, T. .
CHEMICAL ENGINEERING SCIENCE, 2007, 62 (06) :1650-1669
[7]   A chemical and thermodynamic model of oil generation in hydrocarbon source rocks [J].
Helgeson, Harold C. ;
Richard, Laurent ;
McKenzie, William F. ;
Norton, Denis L. ;
Schmitt, Alexandra .
GEOCHIMICA ET COSMOCHIMICA ACTA, 2009, 73 (03) :594-695
[8]   Microbiology of synthesis gas fermentation for biofuel production [J].
Henstra, Anne M. ;
Sipma, Jan ;
Rinzema, Arjen ;
Stams, Alfons J. M. .
CURRENT OPINION IN BIOTECHNOLOGY, 2007, 18 (03) :200-206
[9]   Oxygen mass transfer in a stirred tank bioreactor using different impeller configurations for environmental purposes [J].
Karimi, Ali ;
Golbabaei, Farideh ;
Mehrnia, Momammad Reza ;
Neghab, Masoud ;
Mohammad, Kazem ;
Nikpey, Ahmad ;
Pourmand, Mohammad Reza .
IRANIAN JOURNAL OF ENVIRONMENTAL HEALTH SCIENCE & ENGINEERING, 2013, 10
[10]   EFFECTS OF TEMPERATURE ON METHANE CONSUMPTION IN A FOREST SOIL AND IN PURE CULTURES OF THE METHANOTROPH METHYLOMONAS-RUBRA [J].
KING, GM ;
ADAMSEN, APS .
APPLIED AND ENVIRONMENTAL MICROBIOLOGY, 1992, 58 (09) :2758-2763