Mapping spin-polarized transitions with atomic resolution

被引:44
作者
Schattschneider, P. [1 ,2 ]
Schaffer, B. [3 ,4 ]
Ennen, I. [1 ]
Verbeeck, J. [5 ]
机构
[1] Vienna Univ Technol, Inst Festkorperphys, A-1040 Vienna, Austria
[2] Vienna Univ Technol, Univ Serv Ctr Elect Microscopy, A-1040 Vienna, Austria
[3] STFC Daresbury Labs, SuperSTEM, Warrington WA4 4AD, Cheshire, England
[4] Univ Glasgow, SUPA Sch Phys & Astron, Kelvin Nanocharacterisat Ctr, Glasgow G12 8QQ, Lanark, Scotland
[5] Univ Antwerp, EMAT, B-2020 Antwerp, Belgium
基金
欧洲研究理事会; 奥地利科学基金会;
关键词
ELECTRON-MICROSCOPE; CIRCULAR-DICHROISM; BEAMS; STEM;
D O I
10.1103/PhysRevB.85.134422
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The coupling of angstrom-sized electron probes with spin-polarized electronic transitions shows that the inelastically scattered probe electron is in a mixed state containing electron vortices with nonzero orbital angular momentum. These electrons create an asymmetric intensity distribution in energy filtered diffraction patterns, giving access to maps of the magnetic moments with atomic resolution. A feasibility experiment shows evidence of the predicted effect. Potential applications are column-by-column maps of magnetic ordering, and the creation of angstrom-sized free electrons with orbital angular momentum by inelastic scattering in a thin ferromagnetic foil.
引用
收藏
页数:8
相关论文
共 34 条
[1]   INELASTIC-SCATTERING OF FAST ELECTRONS BY CRYSTALS [J].
ALLEN, LJ ;
JOSEFSSON, TW .
PHYSICAL REVIEW B, 1995, 52 (05) :3184-3198
[2]   Relativistic Electron Vortex Beams: Angular Momentum and Spin-Orbit Interaction [J].
Bliokh, Konstantin Y. ;
Dennis, Mark R. ;
Nori, Franco .
PHYSICAL REVIEW LETTERS, 2011, 107 (17)
[3]   Semiclassical dynamics of electron wave packet states with phase vortices [J].
Bliokh, Konstantin Yu. ;
Bliokh, Yury P. ;
Savel'ev, Sergey ;
Nori, Franco .
PHYSICAL REVIEW LETTERS, 2007, 99 (19)
[4]   Experimental application of sum rules for electron energy loss magnetic chiral dichroism [J].
Calmels, L. ;
Houdellier, F. ;
Warot-Fonrose, B. ;
Gatel, C. ;
Hyetch, M. J. ;
Serin, V. ;
Snoeck, E. .
PHYSICAL REVIEW B, 2007, 76 (06)
[5]   Multiple elastic scattering of core-loss electrons in atomic resolution imaging [J].
Dwyer, C. ;
Findlay, S. D. ;
Allen, L. J. .
PHYSICAL REVIEW B, 2008, 77 (18)
[6]  
Ennen I., 2011, J MAGN MAGN IN PRESS
[7]   Imaging High-Energy Electrons Propagating in a Crystal [J].
Etheridge, Joanne ;
Lazar, Sorin ;
Dwyer, Christian ;
Botton, Gianluigi A. .
PHYSICAL REVIEW LETTERS, 2011, 106 (16)
[8]   Imaging using inelastically scattered electrons in CTEM and STEM geometry [J].
Findlay, S. D. ;
Schattschneider, P. ;
Allen, L. J. .
ULTRAMICROSCOPY, 2007, 108 (01) :58-67
[9]   THE THEORY OF KIKUCHI PATTERNS [J].
KAINUMA, Y .
ACTA CRYSTALLOGRAPHICA, 1955, 8 (05) :247-257
[10]   Direct measurement of ferromagnetic ordering in biaxially strained LaCoO3 thin films [J].
Klie, R. F. ;
Yuan, T. ;
Tanase, M. ;
Yang, G. ;
Ramasse, Q. .
APPLIED PHYSICS LETTERS, 2010, 96 (08)