Production of low-tar producer gas from air gasification of mixed plastic waste in a two-stage gasifier using olivine combined with activated carbon

被引:62
作者
Cho, Min-Hwan [1 ]
Mun, Tae-Young [1 ]
Kim, Joo-Sik [1 ]
机构
[1] Univ Seoul, Dept Energy & Environm Syst Engn, Seoul 130743, South Korea
关键词
Mixed plastic wastes; Two-stage gasifier; Tar removal; Olivine; Activated carbon; Coke; FLUIDIZED-BED GASIFICATION; REMOVAL CATALYST; BIOMASS GASIFIERS;
D O I
10.1016/j.energy.2013.06.021
中图分类号
O414.1 [热力学];
学科分类号
摘要
A fraction of mixed plastic waste was gasified using olivine as a bed material and activated carbon as a tar-cracking additive in a two-stage gasifier. The effects of the amount of activated carbon, the use of an activated carbon filter, and the removal of an EP (electrostatic precipitator) from the process on the gas composition and tar amount generated were investigated. The effects of the ER (equivalence ratio), the type of distributor, the use of steam and the use of a wire mesh basket for activated carbon on the coke removal were also examined. As a result, H-2 concentrations of around 30 vol% were obtained with 1500 g of activated carbon. The tar removal efficiency was maximized at about 98% with the application of 1500 g of activated carbon and steam. The LHVs (lower heating values) of the producer gases obtained with the two additives at ERs of about 0.31 were in the range of 53-6.2 MJ/Nm(3). (C) 2013 Elsevier Ltd. All rights reserved.
引用
收藏
页码:688 / 694
页数:7
相关论文
共 20 条
[1]   Tar removal during the fluidized bed gasification of plastic waste [J].
Arena, Umberto ;
Zaccariello, Lucio ;
Mastellone, Maria Laura .
WASTE MANAGEMENT, 2009, 29 (02) :783-791
[2]   Laboratory evaluation of calcium-, iron-, and potassium-based carbon composite sorbents for capture of hydrogen chloride gas [J].
Bhaskar, T ;
Matsui, T ;
Nitta, K ;
Uddin, MA ;
Muto, AK ;
Sakata, Y .
ENERGY & FUELS, 2002, 16 (06) :1533-1539
[3]   Gasification process of wastes containing PVC [J].
Borgianni, C ;
De Filippis, P ;
Pochetti, F ;
Paolucci, M .
FUEL, 2002, 81 (14) :1827-1833
[4]   Air gasification of mixed plastic wastes using calcined dolomite and activated carbon in a two-stage gasifier to reduce tar [J].
Cho, Min-Hwan ;
Mun, Tae-Young ;
Kim, Joo-Sik .
ENERGY, 2013, 53 :299-305
[5]   Olivine as tar removal catalyst for biomass gasifiers:: Catalyst characterization [J].
Devi, L ;
Craje, M ;
Thüne, P ;
Ptasinski, KJ ;
Janssen, FJJG .
APPLIED CATALYSIS A-GENERAL, 2005, 294 (01) :68-79
[6]   Pretreated olivine as tar removal catalyst for biomass gasifiers: investigation using naphthalene as model biomass tar [J].
Devi, L ;
Ptasinski, KJ ;
Janssen, FJJG .
FUEL PROCESSING TECHNOLOGY, 2005, 86 (06) :707-730
[7]   Olivine as a tar removal catalyst during fluidized bed gasification of plastic waste [J].
Mastellone, Maria Laura ;
Arena, Umberto .
AICHE JOURNAL, 2008, 54 (06) :1656-1667
[8]   Co-gasification of coal, plastic waste and wood in a bubbling fluidized bed reactor [J].
Mastellone, Maria Laura ;
Zaccariello, Lucio ;
Arena, Umberto .
FUEL, 2010, 89 (10) :2991-3000
[9]   Tar formation in a steam-O2 blown CFB gasifier and a steam blown PBFB gasifier (BabyHPR): Comparison between different on-line measurement techniques and the off-line SPA sampling and analysis method [J].
Meng, Xiangmei ;
Mitsakis, Panagiotis ;
Mayerhofer, Matthias ;
de Jong, Wiebren ;
Gaderer, Matthias ;
Verkooijen, Adrian H. M. ;
Spliethoff, Hartmut .
FUEL PROCESSING TECHNOLOGY, 2012, 100 :16-29
[10]   Air gasification of dried sewage sludge in a two-stage gasifier: Part 1. The effects and reusability of additives on the removal of tar and hydrogen production [J].
Mun, Tae-Young ;
Kim, Jin-Won ;
Kim, Joo-Sik .
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2013, 38 (13) :5226-5234