Multi-color fluorescent carbon dots with single wavelength excitation for white light-emitting diodes

被引:61
作者
Zhao, Kangxu [1 ]
Zheng, Xuan [1 ]
Zhang, Huijun [1 ]
Xu, Menghan [1 ]
Wang, Shan [1 ]
Yang, Quanling [1 ]
Xiong, Chuanxi [1 ]
机构
[1] Wuhan Univ Technol, State Key Lab Adv Technol Mat Synth & Proc, Sch Mat Sci & Engn, Wuhan 430070, Hubei, Peoples R China
基金
中国国家自然科学基金;
关键词
Carbon dots; Solvothermal; Photoluminescence; Excitation-independent; Optoelectronic applications; GRAPHENE QUANTUM DOTS; FULL-COLOR EMISSION; OPTICAL-PROPERTIES; BLUE LUMINESCENCE; PHOTOLUMINESCENCE; RED; RECOMBINATION; PH;
D O I
10.1016/j.jallcom.2019.04.146
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Carbon dots (CDs) have been applied in numerous fields by virtue of their excellent features. Multi-color fluorescent carbon dots with high photoluminescence (PL) quantum yield are still the emphases for research. Here, by using 3,5-diaminobenzoic acid and 3,4-diaminobenzoic acid, multi-color-red, green, blue (RGB) emitting CDs (RGB-CDs) were successfully synthesized via a one-pot solvothermal route. The RGB-CDs exhibited stable optical properties and significant photoluminescence characteristics with excitation-independent. Structure and element analysis indicated that conjugated graphite structure of carbon cores and oxygen on surface states were responsible for the RGB color emissions of carbon dots. Moreover, RGB-color and white light-emitting diodes (LEDs) were fabricated by these multi-color fluorescent carbon dots. The LEDs exhibited excellent lighting performance, indicating that these RGB-CDs have the potential to substitute rare elements for solid-state optoelectronic applications. (C) 2019 Elsevier B.V. All rights reserved.
引用
收藏
页码:613 / 619
页数:7
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