Carbon neutral hydrocarbons

被引:86
作者
Zeman, Frank S. [1 ]
Keith, David W. [2 ,3 ]
机构
[1] Columbia Univ, Dept Earth & Environm Engn, New York, NY 10027 USA
[2] Univ Calgary, Dept Chem & Petr Engn, Calgary, AB T2N 1N4, Canada
[3] Univ Calgary, Dept Econ, Calgary, AB T2N 1N4, Canada
来源
PHILOSOPHICAL TRANSACTIONS OF THE ROYAL SOCIETY A-MATHEMATICAL PHYSICAL AND ENGINEERING SCIENCES | 2008年 / 366卷 / 1882期
关键词
air capture; transportation; hydrocarbons; mitigation; hydrogen;
D O I
10.1098/rsta.2008.0143
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Reducing greenhouse gas emissions from the transportation sector may be the most difficult aspect of climate change mitigation. We suggest that carbon neutral hydrocarbons (CNHCs) offer an alternative pathway for deep emission cuts that complement the use of decarbonized energy carriers. Such fuels are synthesized from atmospheric carbon dioxide (CO2) and carbon neutral hydrogen. The result is a liquid fuel compatible with the existing transportation infrastructure and therefore capable of a gradual deployment with minimum supply disruption. Capturing the atmospheric CO2 can be accomplished using biomass or industrial methods referred to as air capture. The viability of biomass fuels is strongly dependent on the environmental impacts of biomass production. Strong constraints on land use may favour the use of air capture. We conclude that CNHCs may be a viable alternative to hydrogen or conventional biofuels and warrant a comparable level of research effort and support.
引用
收藏
页码:3901 / 3918
页数:18
相关论文
共 44 条
[1]   Sustainable fuel for the transportation sector [J].
Agrawal, Rakesh ;
Singh, Navneet R. ;
Ribeiro, Fabio H. ;
Delgass, W. Nicholas .
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2007, 104 (12) :4828-4833
[2]  
[Anonymous], 1998, LIME LIMESTONE CHEM
[3]  
[Anonymous], CONTR WORK GROUP 3 4
[4]  
AUDUS H, 2004, P 7 INT C GREENH GAS, V1, P187
[5]   Process design and energy requirements for the capture of carbon dioxide from air [J].
Baciocchi, Renato ;
Storti, Giuseppe ;
Mazzotti, Marco .
CHEMICAL ENGINEERING AND PROCESSING-PROCESS INTENSIFICATION, 2006, 45 (12) :1047-1058
[6]   CO2 RECYCLING FOR HYDROGEN STORAGE AND TRANSPORTATION - ELECTROCHEMICAL CO2 REMOVAL AND FIXATION [J].
BANDI, A ;
SPECHT, M ;
WEIMER, T ;
SCHABER, K .
ENERGY CONVERSION AND MANAGEMENT, 1995, 36 (6-9) :899-902
[7]   Coping with carbon: a near-term strategy to limit carbon dioxide emissions from power stations [J].
Breeze, Paul .
PHILOSOPHICAL TRANSACTIONS OF THE ROYAL SOCIETY A-MATHEMATICAL PHYSICAL AND ENGINEERING SCIENCES, 2008, 366 (1882) :3891-3900
[8]   Renewable hydrogen utilisation for the production of methanol [J].
Cifre, P. Galindo ;
Badr, O. .
ENERGY CONVERSION AND MANAGEMENT, 2007, 48 (02) :519-527
[9]  
EPA United States Environmental Protection Agency, 2005, EPA420F05001
[10]   Cost to produce and deliver switchgrass biomass to an ethanol-conversion facility in the Southern Plains of the United States [J].
Epplin, FM .
BIOMASS & BIOENERGY, 1996, 11 (06) :459-467