MXene-Coated Mesh Membrane with Underwater Superoleophobicity for High-efficiency Oil-water Separation

被引:5
|
作者
Zhang Jianhui [1 ]
Zhou Jinya [1 ]
Lin Haibo [1 ,2 ]
Li Zhan [2 ]
Fang Qianrong [1 ,2 ]
Xue Ming [1 ,2 ]
Qiu Shilun [1 ,2 ]
机构
[1] Jilin Univ, Zhuhai Coll, Zhuhai 519041, Peoples R China
[2] Jilin Univ, Coll Chem, Changchun 130012, Jilin, Peoples R China
来源
CHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE | 2019年 / 40卷 / 04期
基金
中国国家自然科学基金;
关键词
2D nanosheet; MXene-coated mesh membrane; Underwater superoleophobicity; Oil-water separation; OIL/WATER SEPARATION; NEXT-GENERATION; CLEANUP; FILM;
D O I
10.7503/cjcu20190025
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Owing to the hydrophilicity and flake-like structure of the two-dimensional (2D) MXene (Ti3C2Tx), the 2D MXene nanosheets were coated onto the stainless steel mesh to fabricate a novel hydrophilic and underwater superoleophobic mesh membrane with a corrugated micro- and nanostructure surface. For a series of oil-water mixtures, the MXene-caoted mesh membrane can achieve gravity-driven high-efficiency oil-water separation with excellent separation efficiency of over 99.99% , residual oil content of less than 4 mg/L in collected water, and water flux up to 57. 52 L . m(-2) . s(-1). In addition, MXene-coated mesh membranes display outstanding stability and cycleability.
引用
收藏
页码:624 / 631
页数:8
相关论文
共 42 条
  • [1] Interfacial microfluidic processing of metal-organic framework hollow fiber membranes
    Brown, Andrew J.
    Brunelli, Nicholas A.
    Eum, Kiwon
    Rashidi, Fereshteh
    Johnson, J. R.
    Koros, William J.
    Jones, Christopher W.
    Nair, Sankar
    [J]. SCIENCE, 2014, 345 (6192) : 72 - 75
  • [2] Wettability of porous surfaces.
    Cassie, ABD
    Baxter, S
    [J]. TRANSACTIONS OF THE FARADAY SOCIETY, 1944, 40 : 0546 - 0550
  • [3] Ion sieving in graphene oxide membranes via cationic control of interlayer spacing
    Chen, Liang
    Shi, Guosheng
    Shen, Jie
    Peng, Bingquan
    Zhang, Bowu
    Wang, Yuzhu
    Bian, Fenggang
    Wang, Jiajun
    Li, Deyuan
    Qian, Zhe
    Xu, Gang
    Liu, Gongping
    Zeng, Jianrong
    Zhang, Lijuan
    Yang, Yizhou
    Zhou, Guoquan
    Wu, Minghong
    Jin, Wanqin
    Li, Jingye
    Fang, Haiping
    [J]. NATURE, 2017, 550 (7676) : 415 - 418
  • [4] Oil/Water Separation with Selective Superantiwetting/Superwetting Surface Materials
    Chu, Zonglin
    Feng, Yujun
    Seeger, Stefan
    [J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2015, 54 (08) : 2328 - 2338
  • [5] Ding L, 2017, Angew. Chem. Int. Ed, V129, P1851, DOI [DOI 10.1002/ANGE.201609306, 10.1002/ANGE.201609306]
  • [6] MXene molecular sieving membranes for highly efficient gas separation
    Ding, Li
    Wei, Yanying
    Li, Libo
    Zhang, Tao
    Wang, Haihui
    Xue, Jian
    Ding, Liang-Xin
    Wang, Suqing
    Caro, Juergen
    Gogotsi, Yury
    [J]. NATURE COMMUNICATIONS, 2018, 9
  • [7] Continuous, High-Speed, and Efficient Oil/Water Separation using Meshes with Antagonistic Wetting Properties
    Dunderdale, Gary J.
    Urata, Chihiro
    Sato, Tomoya
    England, Matt W.
    Hozumi, Atsushi
    [J]. ACS APPLIED MATERIALS & INTERFACES, 2015, 7 (34) : 18915 - 18919
  • [8] A super-hydrophobic and super-oleophilic coating mesh film for the separation of oil and water
    Feng, L
    Zhang, ZY
    Mai, ZH
    Ma, YM
    Liu, BQ
    Jiang, L
    Zhu, DB
    [J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2004, 43 (15) : 2012 - 2014
  • [9] Super-hydrophobic surfaces: From natural to artificial
    Feng, L
    Li, SH
    Li, YS
    Li, HJ
    Zhang, LJ
    Zhai, J
    Song, YL
    Liu, BQ
    Jiang, L
    Zhu, DB
    [J]. ADVANCED MATERIALS, 2002, 14 (24) : 1857 - 1860
  • [10] Separation of oil and water in oil spill recovery operations
    Gaaseidnes, K
    Turbeville, J
    [J]. PURE AND APPLIED CHEMISTRY, 1999, 71 (01) : 95 - 101