Morphology control of tunneling dielectric towards high-performance organic field-effect transistor nonvolatile memory

被引:49
作者
She, Xiao-Jian [1 ]
Liu, Chang-Hai [1 ]
Sun, Qi-Jun [1 ]
Gao, Xu [1 ]
Wang, Sui-Dong [1 ]
机构
[1] Soochow Univ, Inst Funct Nano & Soft Mat FUNSOM, Jiangsu Key Lab Carbon Based Funct Mat & Devices, Suzhou 215123, Jiangsu, Peoples R China
基金
中国国家自然科学基金;
关键词
Organic field-effect transistors; Nonvolatile memory; Floating gate; Au nanoparticles; Polystyrene; Pentacene; THIN-FILM; POLYMER; HYSTERESIS; STORAGE; VOLTAGE; DEVICES; GOLD;
D O I
10.1016/j.orgel.2012.05.051
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We report high-performance organic field-effect transistor nonvolatile memory based on nano-floating-gate, which shows a large memory window of about 70 V, high ON/OFF ratio of reading current over 105 after 1 week storage, high field-effect mobility of 0.6 cm(2)/V s, and good programming/erasing/reading endurance. The devices incorporate Au nanoparticles and polystyrene layer on top to form the nano-floating-gate, and we demonstrate that the morphology control of the tunneling dielectric is critically significant to improve the memory performance. The optimized tunneling dielectric morphology is favorable to the efficient charge tunneling, reliable charge storage and high-quality organic film growth. (C) 2012 Elsevier B.V. All rights reserved.
引用
收藏
页码:1908 / 1915
页数:8
相关论文
共 28 条
[1]   Organic non-volatile memory based on pentacene field-effect transistors using a polymeric gate electret [J].
Baeg, Kang-Jun ;
Noh, Yong-Young ;
Ghim, Jieun ;
Kang, Seok-Ju ;
Lee, Hyemi ;
Kim, Dong-Yu .
ADVANCED MATERIALS, 2006, 18 (23) :3179-+
[2]   Controllable Shifts in Threshold Voltage of Top-Gate Polymer Field-Effect Transistors for Applications in Organic Nano Floating Gate Memory [J].
Baeg, Kang-Jun ;
Noh, Yong-Young ;
Sirringhaus, Henning ;
Kim, Dong-Yu .
ADVANCED FUNCTIONAL MATERIALS, 2010, 20 (02) :224-230
[3]   Concept of a Molecular Charge Storage Dielectric Layer for Organic Thin-Film Memory Transistors [J].
Burkhardt, Martin ;
Jedaa, Abdesselam ;
Novak, Michael ;
Ebel, Alexander ;
Voitchovsky, Kislon ;
Stellacci, Francesco ;
Hirsch, Andreas ;
Halik, Marcus .
ADVANCED MATERIALS, 2010, 22 (23) :2525-2528
[4]   An organic charge trapping memory transistor with bottom source and drain contacts [J].
Debucquoy, Maarten ;
Bode, Dieter ;
Genoe, Jan ;
Gelinck, Gerwin H. ;
Heremans, Paul .
APPLIED PHYSICS LETTERS, 2009, 95 (10)
[5]   High-performance organic field-effect transistors with low-cost copper electrodes [J].
Di, Chong-an ;
Yu, Gui ;
Liu, Yunqi ;
Guo, Yunlong ;
Wang, Ying ;
Wu, Weiping ;
Zhu, Daoben .
ADVANCED MATERIALS, 2008, 20 (07) :1286-+
[6]   Mobile ionic impurities in poly(vinyl alcohol) gate dielectric:: Possible source of the hysteresis in organic field-effect transistors [J].
Egginger, Martin ;
Irimia-Vladu, Mihai ;
Schwoediauer, Reinhard ;
Tanda, Andreas ;
Frischauf, Irene ;
Bauer, Siegfried ;
Sariciftci, Niyazi Serdar .
ADVANCED MATERIALS, 2008, 20 (05) :1018-+
[7]   Current versus gate voltage hysteresis in organic field effect transistors [J].
Egginger, Martin ;
Bauer, Siegfried ;
Schwoediauer, Reinhard ;
Neugebauer, Helmut ;
Sariciftci, Niyazi Serdar .
MONATSHEFTE FUR CHEMIE, 2009, 140 (07) :735-750
[8]   Functional Organic Field-Effect Transistors [J].
Guo, Yunlong ;
Yu, Gui ;
Liu, Yunqi .
ADVANCED MATERIALS, 2010, 22 (40) :4427-4447
[9]   Multibit Storage of Organic Thin-Film Field-Effect Transistors [J].
Guo, Yunlong ;
Di, Chong-an ;
Ye, Shanghui ;
Sun, Xiangnan ;
Zheng, Jian ;
Wen, Yugeng ;
Wu, Weiping ;
Yu, Gui ;
Liu, Yunqi .
ADVANCED MATERIALS, 2009, 21 (19) :1954-1959
[10]   Nanoparticle size dependent threshold voltage shifts in organic memory transistors [J].
Han, Su-Ting ;
Zhou, Ye ;
Xu, Zong-Xiang ;
Roy, V. A. L. ;
Hung, T. F. .
JOURNAL OF MATERIALS CHEMISTRY, 2011, 21 (38) :14575-14580