A bowl-shaped molecule for organic field-effect transistors: crystal engineering and charge transport switching by oxygen doping

被引：110

作者：

Shi, Ke ^{[1
]}

Lei, Ting ^{[1
]}

Wang, Xiao-Ye ^{[1
]}

Wang, Jie-Yu ^{[1
]}

Pei, Jian ^{[1
]}

机构：

[1] Peking Univ, Coll Chem & Mol Engn, Beijing Natl Lab Mol Sci, Key Lab Bioorgan Chem & Mol Engn,Minist Educ, Beijing 100871, Peoples R China

来源：

CHEMICAL SCIENCE | 2014年 / 5卷 / 03期

基金：

中国国家自然科学基金;

关键词：

N-TYPE; STRUCTURAL-ANALYSIS; CORANNULENE; POLYMER; MOBILITY; SEMICONDUCTORS; HYDROCARBONS; DERIVATIVES; BUCKYBOWL; FRAGMENTS;

D O I：

10.1039/c3sc52701h

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

A corannulene-based derivative was facilely developed with a bowl-shaped structure. Highly ordered cofacial convex-concave stacking was realized through tuning the molecular dipoles, which is favorable for charge transport. Organic field-effect transistors were fabricated, providing opportunities for a broad class of corannulene derivatives and buckybowl aromatics for application in future organic electronic devices.

引用

收藏

页码：1041 / 1045

页数：5

相关论文

共 42 条

[1]

[Anonymous], 2012, ANGEW CHEM

[2] Corannulene-based fullerene fragments C20H10-C50H10: when does a buckybowl become a buckytube? [J].

Baldridge, KK ;

Siegel, JS .

THEORETICAL CHEMISTRY ACCOUNTS, 1997, 97 (1-4) :67-71

[3] Molecular Design and Ordering Effects in π-Functional Materials for Transistor and Solar Cell Applications [J].

Beaujuge, Pierre M. ;

Frechet, Jean M. J. .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2011, 133 (50) :20009-20029

[4] Electrochemical and Theoretical Investigation of Corannulene Reduction Processes [J].

Bruno, Carlo ;

Benassi, Rois ;

Passalacqua, Alessio ;

Paolucci, Francesco ;

Fontanesi, Claudio ;

Marcaccio, Massimo ;

Jackson, Edward A. ;

Scott, Lawrence T. .

JOURNAL OF PHYSICAL CHEMISTRY B, 2009, 113 (07) :1954-1962

[5] Highly p-Extended Copolymers with Diketopyrrolopyrrole Moieties for High-Performance Field-Effect Transistors [J].

Chen, Huajie ;

Guo, Yunlong ;

Yu, Gui ;

Zhao, Yan ;

Zhang, Ji ;

Gao, Dong ;

Liu, Hongtao ;

Liu, Yunqi .

ADVANCED MATERIALS, 2012, 24 (34) :4618-4622

[6] Shape-shifting in contorted dibenzotetrathienocoronenes [J].

Chiu, Chien-Yang ;

Kim, Bumjung ;

Gorodetsky, Alon A. ;

Sattler, Wesley ;

Wei, Sujun ;

Sattler, Aaron ;

Steigerwald, Michael ;

Nuckolls, Colin .

CHEMICAL SCIENCE, 2011, 2 (08) :1480-1486

[7] Bulk Heterojunction Solar Cells Using Thieno[3,4-c]pyrrole-4,6-dione and Dithieno[3,2-b:2′,3′-d]silole Copolymer with a Power Conversion Efficiency of 7.3% [J].

Chu, Ta-Ya ;

Lu, Jianping ;

Beaupre, Serge ;

Zhang, Yanguang ;

Pouliot, Jean-Remi ;

Wakim, Salem ;

Zhou, Jiayun ;

Leclerc, Mario ;

Li, Zhao ;

Ding, Jianfu ;

Tao, Ye .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2011, 133 (12) :4250-4253

[8] High Resolution Optical Spectroscopy of Air-Induced Electrical Instabilities in n-type Polymer Semiconductors [J].

Di Pietro, Riccardo ;

Sirringhaus, Henning .

ADVANCED MATERIALS, 2012, 24 (25) :3367-3372

[9] Alkylene-Chain Effect on Microwire Growth and Crystal Packing of π-Moieties [J].

Ding, Lin ;

Li, Hai-Bin ;

Lei, Ting ;

Ying, Han-Ze ;

Wang, Rui-Bo ;

Zhou, Yan ;

Su, Zhong-Min ;

Pei, Jian .

CHEMISTRY OF MATERIALS, 2012, 24 (10) :1944-1949

[10] CRYSTAL AND MOLECULAR-STRUCTURE OF CORANNULENE, C-20H-10 [J].

HANSON, JC ;

NORDMAN, CE .

ACTA CRYSTALLOGRAPHICA SECTION B-STRUCTURAL SCIENCE, 1976, 32 (APR15) :1147-1153

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