Bulk electronic structure of Zn-Mg-Y and Zn-Mg-Dy icosahedral quasicrystals

被引:15
作者
Nayak, J. [1 ]
Maniraj, M. [1 ]
Gloskovskii, A. [2 ]
Krajci, M. [3 ]
Sebastian, S. [4 ,5 ]
Fisher, I. R. [4 ,5 ]
Horn, K. [6 ]
Barman, S. R. [1 ]
机构
[1] UGC DAE Consortium Sci Res, Indore 452001, Madhya Pradesh, India
[2] DESY, D-22607 Hamburg, Germany
[3] Slovak Acad Sci, Inst Phys, SK-84511 Bratislava, Slovakia
[4] Stanford Univ, Geballe Lab Adv Mat, Stanford, CA 94305 USA
[5] Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA
[6] Max Planck Gesell, Fritz Haber Inst, D-14195 Berlin, Germany
关键词
DENSITY-OF-STATES; PHOTOELECTRON; PHOTOEMISSION; GROWTH; SPECTROSCOPY; TRANSPORT; SPECTRA; METALS; AUGER; TB;
D O I
10.1103/PhysRevB.91.235116
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We use bulk sensitive hard x-ray photoelectron spectroscopy to provide unambiguous evidence for a pseudogap in the density of states around the Fermi level in icosahedral Zn-Mg-Y and Zn-Mg-Dy quasicrystals, in agreement with our density functional theory calculations. The pseudogap in these Zn-based quasicrystals is less pronounced compared to the Al-based ones such as Al-Pd-Mn and Al-Cu-Fe [J. Nayak et al., Phys. Rev. Lett. 109, 216403 ( 2012)]. This observation is in agreement with transport studies that indicate a larger charge carrier concentration in the Zn-based quasicrystals. Compared to Zn-Mg-Dy, the pseudogap is somewhat deeper in Zn-Mg-Y. The larger width of the Mg 1s and Zn 2p core-level spectra in Zn-Mg-Y is explained by different configurations of the local atomic surrounding compared to Zn-Mg-Dy.
引用
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页数:6
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