Experimental Verification of the Spectral Shift between Near- and Far-Field Peak Intensities of Plasmonic Infrared Nanoantennas

被引:154
作者
Alonso-Gonzalez, P. [1 ]
Albella, P. [1 ,2 ,3 ]
Neubrech, F. [4 ]
Huck, C. [4 ]
Chen, J. [1 ,2 ,3 ]
Golmar, F. [1 ,5 ]
Casanova, F. [1 ,6 ]
Hueso, L. E. [1 ,6 ]
Pucci, A. [4 ]
Aizpurua, J. [2 ,3 ]
Hillenbrand, R. [1 ,6 ]
机构
[1] CIC NanoGUNE, Donostia San Sebastian 20018, Spain
[2] Ctr Fis Mat CSIC UPV EHU, Donostia San Sebastian 20018, Spain
[3] DIPC, Donostia San Sebastian 20018, Spain
[4] Heidelberg Univ, Kirchhoff Inst Phys, D-69120 Heidelberg, Germany
[5] INTI CONICET, San Martin, Bs As, Argentina
[6] Basque Fdn Sci, IKERBASQUE, Bilbao 48011, Spain
关键词
NEAR-FIELD; SURFACE; SCATTERING; MODES; RESONANCES; MOLECULES; NANOPARTICLES; INTERFERENCE; SPECTROSCOPY; SPACE;
D O I
10.1103/PhysRevLett.110.203902
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Theory predicts a distinct spectral shift between the near- and far-field optical response of plasmonic antennas. Here we combine near- field optical microscopy and far-field spectroscopy of individual infrared-resonant nanoantennas to verify experimentally this spectral shift. Numerical calculations corroborate our experimental results. We furthermore discuss the implications of this effect in surface-enhanced infrared spectroscopy.
引用
收藏
页数:6
相关论文
共 51 条
[21]   Transition from Isolated to Collective Modes in Plasmonic Oligomers [J].
Hentschel, Mario ;
Saliba, Michael ;
Vogelgesang, Ralf ;
Giessen, Harald ;
Alivisatos, A. Paul ;
Liu, Na .
NANO LETTERS, 2010, 10 (07) :2721-2726
[22]   Optical oscillation modes of plasmon particles observed in direct space by phase-contrast near-field microscopy [J].
Hillenbrand, R ;
Keilmann, F .
APPLIED PHYSICS B-LASERS AND OPTICS, 2001, 73 (03) :239-243
[23]   SURFACE RAMAN SPECTROELECTROCHEMISTRY .1. HETEROCYCLIC, AROMATIC, AND ALIPHATIC-AMINES ADSORBED ON ANODIZED SILVER ELECTRODE [J].
JEANMAIRE, DL ;
VANDUYNE, RP .
JOURNAL OF ELECTROANALYTICAL CHEMISTRY, 1977, 84 (01) :1-20
[24]   Effect of radiation damping on the spectral response of plasmonic components [J].
Kats, Mikhail A. ;
Yu, Nanfang ;
Genevet, Patrice ;
Gaburro, Zeno ;
Capasso, Federico .
OPTICS EXPRESS, 2011, 19 (22) :21748-21753
[25]   Single molecule detection using surface-enhanced Raman scattering (SERS) [J].
Kneipp, K ;
Wang, Y ;
Kneipp, H ;
Perelman, LT ;
Itzkan, I ;
Dasari, R ;
Feld, MS .
PHYSICAL REVIEW LETTERS, 1997, 78 (09) :1667-1670
[26]   Photodetection with Active Optical Antennas [J].
Knight, Mark W. ;
Sobhani, Heidar ;
Nordlander, Peter ;
Halas, Naomi J. .
SCIENCE, 2011, 332 (6030) :702-704
[27]   Enhancement of single-molecule fluorescence using a gold nanoparticle as an optical nanoantenna [J].
Kuehn, Sergei ;
Hakanson, Ulf ;
Rogobete, Lavinia ;
Sandoghdar, Vahid .
PHYSICAL REVIEW LETTERS, 2006, 97 (01)
[28]   Wavelength-scanned surface-enhanced Raman excitation spectroscopy [J].
McFarland, AD ;
Young, MA ;
Dieringer, JA ;
Van Duyne, RP .
JOURNAL OF PHYSICAL CHEMISTRY B, 2005, 109 (22) :11279-11285
[29]   LOCAL-FIELDS AT THE SURFACE OF NOBLE-METAL MICROSPHERES [J].
MESSINGER, BJ ;
VONRABEN, KU ;
CHANG, RK ;
BARBER, PW .
PHYSICAL REVIEW B, 1981, 24 (02) :649-657
[30]   SURFACE-ENHANCED SPECTROSCOPY [J].
MOSKOVITS, M .
REVIEWS OF MODERN PHYSICS, 1985, 57 (03) :783-826