134Cs and 137CS activities in coastal seawater along Northern Sanriku and Tsugaru Strait, northeastern Japan, after Fukushima Dai-ichi Nuclear Power Plant accident

被引:47
作者
Inoue, M. [1 ]
Kofuji, H. [2 ]
Hamajima, Y. [1 ]
Nagao, S. [1 ]
Yoshida, K. [1 ]
Yamamoto, M. [1 ]
机构
[1] Kanazawa Univ, Low Level Radioact Lab, Inst Nat & Environm Technol, Nomi, Ishikawa 9231224, Japan
[2] Japan Marine Sci Fdn, Minato Ku, Mutsu, Aomori 0350064, Japan
关键词
Cs-134; Cs-137; Coastal seawater; Northern Sanriku; Fukushima Dai-ichi Nuclear Power Plant accident;
D O I
10.1016/j.jenvrad.2011.09.012
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
A total of 37 seawater samples were collected at 10 sites along the coastline of the Northern Sanriku and Tsugaru Strait, 250-450 km north of the Fukushima Dai-ichi Nuclear Power Plant in April-December 2009 and May June 2011, and analyzed for Cs-134 and Cs-137 activities using low-background gamma-spectrometry. The Cs-134 and Cs-137 activities measured in these samples in May 2011 were found to be 2-3 mBq/L and 2.5-4 mBq/L, respectively. By June, these values had decreased by 25-45%/month and 5-30%/month, respectively. These results can be plausibly explained by surface infusion of these isotopes into the sea by atmospheric transport from Fukushima and their subsequent reduction by water migration to off-shore and deeper regions. (C) 2011 Elsevier Ltd. All rights reserved.
引用
收藏
页码:116 / 119
页数:4
相关论文
共 11 条
[1]  
Aomori Prefectural Government, 2011, RAD MEAS RES ENV SAM
[2]   Low level 137Cs measurements in deep seawater samples [J].
Aoyama, M ;
Hirose, K ;
Miyao, T ;
Igarashi, Y .
APPLIED RADIATION AND ISOTOPES, 2000, 53 (1-2) :159-162
[3]  
Araujo, 2009, INAC 2009 INT NUCL A
[4]  
Emergency Operations Center Ministry of Education Culture Sports Science and Technology in Japan, 2011, READ ENV RAD LEV
[5]   Background components of Ge detectors in Ogoya underground laboratory [J].
Hamajima, Y ;
Komura, K .
APPLIED RADIATION AND ISOTOPES, 2004, 61 (2-3) :179-183
[6]   Temporal variations of 90Sr and 137Cs concentrations in Japanese coastal surface seawater and sediments from 1974 to 1998 [J].
Ikeuchi, Y .
DEEP-SEA RESEARCH PART II-TOPICAL STUDIES IN OCEANOGRAPHY, 2003, 50 (17-21) :2713-2726
[7]  
Ministry of Education Culture Sports Science and Technology, 2011, MON INF ENV RAD LEV
[8]  
Ministry of Education Culture Sports Science and Technology in Japan, 1982, MIN ED CULT SPORTS S, V13
[9]   Simple coprecipitation method combined with low-background γ-spectrometry:: Determination of 7Be, 137CS, 210Pb, and radium and thorium isotopes in small-volume coastal water samples [J].
Nakano, Yusuke ;
Inoue, Mutsuo ;
Komura, Kazuhisa .
JOURNAL OF OCEANOGRAPHY, 2008, 64 (05) :713-717
[10]  
Nishida Y., 2003, Oceanogr. Jpn., V12, P487, DOI DOI 10.5928/kaiyou.12.487