Metallic fast reactor fuel fabrication for the global nuclear energy partnership

被引:30
作者
Burkes, Douglas E. [1 ]
Fielding, Randall S. [1 ]
Porter, Douglas L. [1 ]
机构
[1] Idaho Natl Lab, Nucl Fuels & Mat Div, Idaho Falls, ID 83415 USA
关键词
VAPOR PRESSURE; EBR-II; PLUTONIUM; NEPTUNIUM;
D O I
10.1016/j.jnucmat.2009.03.009
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Fast reactors are once again being considered for nuclear power generation, in addition to transmutation of long-lived fission products resident in spent nuclear fuels. This re-consideration follows with intense developmental programs for both fuel and reactor design. One of the two leading candidates for next generation fast reactor fuel is metal alloys, resulting primarily from the successes achieved in the 1960s to early 1990s with both the experimental breeding reactor-II and the fast flux test facility. The goal of the current program is to develop and qualify a nuclear fuel system that performs all of the functions of a conventional, fast-spectrum nuclear fuel while destroying recycled actinides, thereby closing the nuclear fuel cycle. In order to meet this goal, the program must develop efficient and safe fuel fabrication processes designed for remote operation. This paper provides an overview of advanced casting processes investigated in the past, and the development of a gaseous diffusion calculation that demonstrates how straightforward process parameter modification can mitigate the loss of volatile minor actinides in the metal alloy melt. (C) 2009 Elsevier B.V. All rights reserved.
引用
收藏
页码:158 / 163
页数:6
相关论文
共 30 条
[1]   THERMODYNAMICS OF VAPORIZATION OF NEPTUNIUM AND PLUTONIUM [J].
ACKERMANN, RJ ;
RAUH, EG .
JOURNAL OF CHEMICAL THERMODYNAMICS, 1975, 7 (03) :211-218
[2]  
[Anonymous], 2002, A Technology Roadmap for Generation IV Nuclear Energy Systems
[3]  
BURRIS L, 1987, AICHE S SER, V83, P135
[4]   THE VAPOR PRESSURE OF AMERICIUM METAL [J].
CARNIGLIA, SC ;
CUNNINGHAM, BB .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1955, 77 (06) :1502-1502
[5]   THE INTEGRAL FAST-REACTOR [J].
CHANG, YI .
NUCLEAR TECHNOLOGY, 1989, 88 (02) :129-138
[6]   Fuels for sodium-cooled fast reactors: US perspective [J].
Crawford, Douglas C. ;
Porter, Douglas L. ;
Hayes, Steven L. .
JOURNAL OF NUCLEAR MATERIALS, 2007, 371 (1-3) :202-231
[7]   VAPOR PRESSURE OF NEPTUNIUM [J].
EICK, HA ;
MULFORD, RNR .
JOURNAL OF CHEMICAL PHYSICS, 1964, 41 (05) :1475-&
[8]   THE VAPOR PRESSURE OF AMERICIUM [J].
ERWAY, ND ;
SIMPSON, OC .
JOURNAL OF CHEMICAL PHYSICS, 1950, 18 (07) :953-957
[9]   BINARY GASEOUS-DIFFUSION COEFFICIENTS OF MERCURY AND OF ZINC IN HYDROGEN, HELIUM, ARGON, NITROGEN, AND CARBON-DIOXIDE [J].
GARDNER, PJ ;
PANG, P ;
PRESTON, SR .
JOURNAL OF CHEMICAL AND ENGINEERING DATA, 1991, 36 (03) :265-268
[10]  
*ID NAT LAB, 2007, GNEPAFCFFUELTDRP2007