CFD as a Design Tool for Fixed-Bed Reactors with Small Tube-to-Pellet Diameter Ratio: Now or in the Future?

被引:16
作者
Wehinger, Gregor D. [1 ]
Kraume, Matthias [1 ]
机构
[1] Tech Univ Berlin, Fachgebiet Verfahrenstech, Fraunhoferstr 33-36, D-10587 Berlin, Germany
关键词
CFD; Fixed-bed reactor; Heat transfer; Heterogeneous catalysis; Modeling; CYLINDRICAL PARTICLES; HEAT-TRANSFER; SIMULATIONS; METHANE; STEAM; FLOW; TRANSPORT; PROFILES; KINETICS; DEM;
D O I
10.1002/cite.201600155
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Fixed-bed reactors with small ratio of tube to pellet diameter (D/d(p)=N) are applied especially for highly exothermic or endothermic reactions. In this contribution, aspects of an algorithm-based approach are investigated, which models spatially resolved fixed-bed reactors with small N. This approach is compared with experimental data in terms of bed morphology, resulting velocities, heat transfer, and heterogeneous catalysis. Finally, the question is discussed whether CFD can be applied as a design tool for small N fixed-bed reactors.
引用
收藏
页码:447 / 453
页数:7
相关论文
共 22 条
[1]  
[Anonymous], 2014, STAR CCM V9 06
[2]   A Coupled DEM and CFD Simulation of Flow Field and Pressure Drop in Fixed Bed Reactor with Randomly Packed Catalyst Particles [J].
Bai, Hua ;
Theuerkauf, Joerg ;
Gillis, Paul A. ;
Witt, Paul M. .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2009, 48 (08) :4060-4074
[3]   Kinetics of heterogeneous catalytic reactions: Analysis of reaction schemes [J].
Cortright, RD ;
Dumesic, JA .
ADVANCES IN CATALYSIS, VOL 46, 2001, 46 :161-264
[4]   Surface Reaction Kinetics of Steam- and CO2-Reforming as Well as Oxidation of Methane over Nickel-Based Catalysts [J].
Delgado, Karla Herrera ;
Maier, Lubow ;
Tischer, Steffen ;
Zellner, Alexander ;
Stotz, Henning ;
Deutschmann, Olaf .
CATALYSTS, 2015, 5 (02) :871-904
[5]   Heat transfer in fixed beds at very low (<4) tube-to-particle diameter ratio [J].
Dixon, AG .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 1997, 36 (08) :3053-3064
[6]   3D CFD simulations of steam reforming with resolved intraparticle reaction and gradients [J].
Dixon, Anthony G. ;
Taskin, M. Ertan ;
Stitt, E. Hugh ;
Nijemeisland, Michiel .
CHEMICAL ENGINEERING SCIENCE, 2007, 62 (18-20) :4963-4966
[7]   Flow, Transport, and Reaction Interactions in Shaped Cylindrical Particles for Steam Methane Reforming [J].
Dixon, Anthony G. ;
Boudreau, Justin ;
Rocheleau, Anne ;
Troupel, Alexandre ;
Taskin, M. Ertan ;
Nijemeisland, Michiel ;
Stitt, E. Hugh .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2012, 51 (49) :15839-15854
[8]   Systematic mesh development for 3D CFD simulation of fixed beds: Contact points study [J].
Dixon, Anthony G. ;
Nijemeisland, Michiel ;
Stitt, E. Hugh .
COMPUTERS & CHEMICAL ENGINEERING, 2013, 48 :135-153
[9]   Experimental validation of high Reynolds number CFD simulations of heat transfer in a pilot-scale fixed bed tube [J].
Dixon, Anthony G. ;
Walls, Gregory ;
Stanness, Helen ;
Nijemeisland, Michiel ;
Stitt, E. Hugh .
CHEMICAL ENGINEERING JOURNAL, 2012, 200 :344-356
[10]   DEM-CFD simulations of fixed bed reactors with small tube to particle diameter ratios [J].
Eppinger, T. ;
Seidler, K. ;
Kraume, M. .
CHEMICAL ENGINEERING JOURNAL, 2011, 166 (01) :324-331