A global analysis of climate-relevant aerosol properties retrieved from the network of Global Atmosphere Watch (GAW) near-surface observatories

被引：71

作者：

Laj, Paolo ^{[1
,2
,3
]}

Bigi, Alessandro ^{[4
]}

Rose, Clemence ^{[5
]}

Andrews, Elisabeth ^{[6
,7
]}

Myhre, Cathrine Lund ^{[8
]}

Coen, Martine Collaud ^{[9
]}

Lin, Yong ^{[8
]}

Wiedensohler, Alfred ^{[10
]}

Schulz, Michael ^{[11
]}

Ogren, John A. ^{[7
]}

Fiebig, Markus ^{[8
]}

Gliss, Jonas ^{[11
]}

Mortier, Augustin ^{[11
]}

Pandolfi, Marco ^{[12
]}

Petaja, Tuukka ^{[3
]}

Kim, Sang-Woo ^{[13
]}

Aas, Wenche ^{[8
]}

Putaud, Jean-Philippe ^{[14
]}

Mayol-Bracero, Olga ^{[15
]}

Keywood, Melita ^{[16
]}

Labrador, Lorenzo ^{[17
]}

Aalto, Pasi ^{[3
]}

Ahlberg, Erik ^{[18
]}

Alados Arboledas, Lucas ^{[19
,20
]}

Alastuey, Andres ^{[12
]}

Andrade, Marcos ^{[21
]}

Artinano, Begona ^{[22
]}

Ausmeel, Stina ^{[18
]}

Arsov, Todor ^{[23
]}

Asmi, Eija ^{[24
]}

Backman, John ^{[24
]}

Baltensperger, Urs ^{[25
]}

Bastian, Susanne ^{[26
]}

Bath, Olaf ^{[27
]}

Beukes, Johan Paul ^{[28
]}

Brem, Benjamin T. ^{[25
]}

Bukowiecki, Nicolas ^{[29
]}

Conil, Sebastien ^{[30
]}

Couret, Cedric ^{[27
]}

Day, Derek ^{[31
]}

Dayantolis, Wan ^{[32
]}

Degorska, Anna ^{[33
]}

Eleftheriadis, Konstantinos ^{[34
]}

Fetfatzis, Prodromos ^{[34
]}

Favez, Olivier ^{[35
]}

Flentje, Harald ^{[36
]}

Gini, Maria I. ^{[34
]}

Gregoric, Asta ^{[37
]}

Gysel-Beer, Martin ^{[14
,25
]}

Hallar, A. Gannet ^{[38
]}

机构：

[1] Univ Grenoble Alpes, CNRS, IRD, Grenoble INP,IGE, F-38000 Grenoble, France

[2] Natl Res Council Italy, Inst Atmospher Sci & Climate, Bologna, Italy

[3] Univ Helsinki, Inst Atmospher & Earth Syst Res, Helsinki, Finland

[4] Univ Modena & Reggio Emilia, Dept Engn Enzo Ferrari, Modena, Italy

[5] Univ Clermont Auvergne, CNRS, LaMP, OPGC, Clermont Ferrand, France

[6] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA

[7] NOAA, Earth Syst Res Lab, Boulder, CO USA

[8] NILU Norwegian Inst Air Res, Kjeller, Norway

[9] MeteoSwiss, Fed Off Meteorol & Climatol, Payerne, Switzerland

[10] Inst Tropospher Res, Leipzig, Germany

[11] Norwegian Meteorol Inst, Oslo, Norway

[12] Spanish Res Council CSIC, Inst Environm Assessment & Water Res IDAEA, Barcelona, Spain

[13] Seoul Natl Univ, Sch Earth & Environm Sci, Seoul, South Korea

[14] European Commiss, Joint Res Ctr JRC, Ispra, Italy

[15] Univ Puerto Rico, Rio Piedras Campus, San Juan, PR USA

[16] CSIRO Oceans & Atmosphere, PMB1, Aspendale, Vic, Australia

[17] Global Atmosphere Watch Secretariat, World Meteorol Org, Geneva, Switzerland

[18] Lund Univ, Div Nucl Phys, Dept Phys, POB 118, S-22100 Lund, Sweden

[19] Univ Granada, Dept Appl Phys, Granada, Spain

[20] Univ Granada, Andalusian Inst Earth Syst Res IISTA CEAMA, Autonomous Govt Andalusia, Granada, Spain

[21] Univ Mayor San Andres, Lab Fis Atmosfera, La Paz, Bolivia

[22] CIEMAT, Ctr Res Energy Environm & Technol, CSIC, Joint Res Unit, Madrid, Spain

[23] Bulgarian Acad Sci, Inst Nucl Res & Nucl Energy, Sofia, Bulgaria

[24] Finnish Meteorol Inst, Atmospher Composit Res, Helsinki, Finland

[25] Paul Scherrer Inst, Lab Atmospher Chem, Villigen, Switzerland

[26] Saxon State Off Environm Agr & Geol LfULG, Dresden, Germany

[27] German Environm Agcy UBA, Zugspitze, Germany

[28] North West Univ, Unit Environm Sci & Management, ZA-2520 Potchefstroom, South Africa

[29] Univ Basel, Dept Environm Sci, Atmospher Sci, Basel, Switzerland

[30] GES Observ Perenne Environm, ANDRA DRD, F-55290 Bures, France

[31] Colorado State Univ, Natl Pk Serv, Cooperat Inst Res Atmosphere, Ft Collins, CO 80523 USA

[32] Tech Operat Unit BMKG, Bukit Kototabang Global Atmosphere Watch Stn, Agam, Indonesia

[33] Natl Res Inst, Inst Environm Protect, Warsaw, Poland

[34] Energy & Safety NCSR Demokritos, Inst Nucl & Radiol Sci & Technol, Attiki, Greece

[35] Inst Natl Environm Ind & Risques INER, Verneuil En Halatte, France

[36] Meteorol Observ Hohenpeissenberg, German Weather Serv, Hohenpeissenberg, Germany

[37] Aerosol Doo, Ljubljana 1000, Slovenia

[38] Univ Utah, Dept Atmospher Sci, Salt Lake City, UT 84112 USA

[39] MTA PE Air Chem Res Grp, Veszprem, Hungary

[40] Swiss Fed Labs Mat Sci & Technol, Empa, Dubendorf, Switzerland

[41] IHC, Energy & Resources Inst, Lodhi Rd, New Delhi, India

[42] Univ Crete, Environm Chem Processes Lab ECPL, Iraklion 71003, Crete, Greece

[43] ZAMG Sonnblick Observ, Freisaalweg, A-165020 Salzburg, Austria

[44] Natl Inst Meteorol Sci, Environm Meteorol Res Div, Seogwipo, South Korea

[45] Hydrometeorol Inst Slovenia, Ljubljana, Slovenia

[46] Stockholm Univ, Dept Environm Sci & Analyt Chem ACES, S-10691 Stockholm, Sweden

[47] Stockholm Univ, Bolin Ctr Climate Res, S-10691 Stockholm, Sweden

[48] South African Weather Serv, Res Dept, Stellenbosch, South Africa

[49] Natl Cent Univ, Dept Atmospher Sci, Taoyuan, Taiwan

[50] Univ La Reunion OSUR, Observ Sci, UMS3365, St Denis De La Reunion, France

来源：

ATMOSPHERIC MEASUREMENT TECHNIQUES | 2020年 / 13卷 / 08期

基金：

芬兰科学院; 瑞典研究理事会; 新加坡国家研究基金会;

关键词：

REGIONAL BACKGROUND SITES; FILTER-BASED MEASUREMENTS; VISIBLE-LIGHT ABSORPTION; BLACK CARBON; OPTICAL-PROPERTIES; SIZE DISTRIBUTIONS; PARTICULATE MATTER; PARTICLE NUMBER; ORGANIC AEROSOL; RADIATIVE PROPERTIES;

D O I：

10.5194/amt-13-4353-2020

中图分类号：

P4 [大气科学（气象学）];

学科分类号：

0706 ; 070601 ;

摘要：

Aerosol particles are essential constituents of the Earth's atmosphere, impacting the earth radiation balance directly by scattering and absorbing solar radiation, and indirectly by acting as cloud condensation nuclei. In contrast to most greenhouse gases, aerosol particles have short atmospheric residence times, resulting in a highly heterogeneous distribution in space and time. There is a clear need to document this variability at regional scale through observations involving, in particular, the in situ near-surface segment of the atmospheric observation system. This paper will provide the widest effort so far to document variability of climate-relevant in situ aerosol properties (namely wavelength dependent particle light scattering and absorption coefficients, particle number concentration and particle number size distribution) from all sites connected to the Global Atmosphere Watch network. High-quality data from almost 90 stations worldwide have been collected and controlled for quality and are reported for a reference year in 2017, providing a very extended and robust view of the variability of these variables worldwide. The range of variability observed worldwide for light scattering and absorption coefficients, single-scattering albedo, and particle number concentration are presented together with preliminary information on their long-term trends and comparison with model simulation for the different stations. The scope of the present paper is also to provide the necessary suite of information, including data provision procedures, quality control and analysis, data policy, and usage of the ground-based aerosol measurement network. It delivers to users of the World Data Centre on Aerosol, the required confidence in data products in the form of a fully characterized value chain, including uncertainty estimation and requirements for contributing to the global climate monitoring system.

引用

页码：4353 / 4392

页数：40

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