Gold-Nanorod-Photosensitized Titanium Dioxide with Wide-Range Visible-Light Harvesting Based on Localized Surface Plasmon Resonance

被引:264
作者
Liu, Lequan [1 ,2 ]
Ouyang, Shuxin [1 ,2 ]
Ye, Jinhua [1 ,2 ,3 ]
机构
[1] Natl Inst Mat Sci, Int Ctr Mat Nanoarchitecton WPI MANA, Tsukuba, Ibaraki 3050044, Japan
[2] Natl Inst Mat Sci, Environm Remediat Mat Unit, Tsukuba, Ibaraki 3050044, Japan
[3] Tianjin Univ, TU NIMS Joint Res Ctr, Sch Mat Sci & Engn, Tianjin, Peoples R China
关键词
gold; photocatalysis; surface plasmon resonance; titania; visible light; PHOTOCATALYTIC ACTIVITY; OPTICAL-PROPERTIES; THERMAL-STABILITY; HIGHLY EFFICIENT; METAL; ABSORPTION; WATER; NANOPARTICLES; SOLAR; TIO2;
D O I
10.1002/anie.201300239
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Broadband visible-light harvesting over TiO2 is achieved by introducing gold nanorods (Au NRs) as antennas based on localized surface plasmon resonance. Furthermore, surfactant removal is achieved by an HClO 4 oxidative method. Not only transversal but also longitudinal plasma of Au NRs can induce photooxidation of 2-propanol, which extends the light harvesting to the near-infrared region. Scale bar: 10 nm. Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
引用
收藏
页码:6689 / 6693
页数:5
相关论文
共 50 条
[1]  
[Anonymous], 2003, ANGEW CHEM INT ED, V42, P4908
[2]  
[Anonymous], 2011, ANGEW CHEM INT ED, V50, P10140
[3]  
[Anonymous], 2004, ANGEW CHEM INT ED, V43, P4463
[4]  
[Anonymous], 2003, ANGEW CHEM, DOI DOI 10.1021/NL9035109
[5]   Improved thermal stability of Au nanorods by use of photosensitive layered titanates for gas sensing applications [J].
Antonello, Alessandro ;
Della Gaspera, Enrico ;
Baldauf, Julia ;
Mattei, Giovanni ;
Martucci, Alessandro .
JOURNAL OF MATERIALS CHEMISTRY, 2011, 21 (34) :13074-13078
[6]   Visible-light photocatalysis in nitrogen-doped titanium oxides [J].
Asahi, R ;
Morikawa, T ;
Ohwaki, T ;
Aoki, K ;
Taga, Y .
SCIENCE, 2001, 293 (5528) :269-271
[7]   Plasmon Inducing Effects for Enhanced Photoelectrochemical Water Splitting: X-ray Absorption Approach to Electronic Structures [J].
Chen, Hao Ming ;
Chen, Chih Kai ;
Chen, Chih-Jung ;
Cheng, Liang-Chien ;
Wu, Pin Chieh ;
Cheng, Bo Han ;
Ho, You Zhe ;
Tseng, Ming Lun ;
Hsu, Ying-Ya ;
Chan, Ting-Shan ;
Lee, Jyh-Fu ;
Liu, Ru-Shi ;
Tsai, Din Ping .
ACS NANO, 2012, 6 (08) :7362-7372
[8]  
Chen X., 2008, ANGEW CHEM, V120, P5433, DOI [DOI 10.1002/ANGE.200800602, 10.1002/ange.200800602]
[9]   Visible-light-driven oxidation of organic contaminants in air with gold nanoparticle catalysts on oxide supports [J].
Chen, Xi ;
Zhu, Huai-Yong ;
Zhao, Jin-Cai ;
Zheng, Zhan-Feng ;
Gao, Xue-Ping .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2008, 47 (29) :5353-5356
[10]   Increasing Solar Absorption for Photocatalysis with Black Hydrogenated Titanium Dioxide Nanocrystals [J].
Chen, Xiaobo ;
Liu, Lei ;
Yu, Peter Y. ;
Mao, Samuel S. .
SCIENCE, 2011, 331 (6018) :746-750