Quasielastic helium atom scattering from a two-dimensional gas of Xe atoms on Pt(111)

被引:49
|
作者
Ellis, J [1 ]
Graham, AP
Toennies, JP
机构
[1] Univ E Anglia, Sch Phys, Norwich NR4 7TJ, Norfolk, England
[2] Max Planck Inst Stromungsforsch, D-37073 Gottingen, Germany
关键词
D O I
10.1103/PhysRevLett.82.5072
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Quasielastic helium atom scattering provides direct evidence for a fully mobile two-dimensional gas of Xe atoms on Pt(111) at a coverage of Theta(Xe) = 0.017 and a temperature of T-s = 105 K. Molecular dynamics simulations of the experimental data show that the frictional coupling rate between the Xe atoms and substrate is less than 0.25 ps(-1) and the lateral potential corrugation for single Xe atoms is less than 9.6 meV, which is only 40% of the value previously determined at high coverage.
引用
收藏
页码:5072 / 5075
页数:4
相关论文
共 50 条
  • [1] Quasielastic helium atom scattering measurements of microscopic diffusional dynamics of H and D on the Pt(111) surface
    Graham, AP
    Menzel, A
    Toennies, JP
    JOURNAL OF CHEMICAL PHYSICS, 1999, 111 (04): : 1676 - 1685
  • [2] Quasielastic helium atom scattering measurements of microscopic diffusional dynamics of H and D on the Pt(111) surface
    Graham, Andrew P.
    Menzel, Alexander
    Toennies, J. Peter
    Journal of Chemical Physics, 111 (04):
  • [3] A helium atom scattering study of the adsorption of NO on Pt(111)
    Fouquet, P
    Graham, AP
    Witte, G
    JOURNAL OF CHEMICAL PHYSICS, 2000, 112 (17): : 7600 - 7605
  • [4] DIRECT EVIDENCE FOR TWO-DIMENSIONAL XE GAS-SOLID PHASE-TRANSITION ON PT(111) BY MEANS OF THERMAL HE SCATTERING
    POELSEMA, B
    VERHEIJ, LK
    COMSA, G
    PHYSICAL REVIEW LETTERS, 1983, 51 (26) : 2410 - 2413
  • [5] TWO-DIMENSIONAL GAS PHASES OF AR, KR, AND XE ON AG(111)
    UNGURIS, J
    BRUCH, LW
    WEBB, MB
    PHILLIPS, JM
    SURFACE SCIENCE, 1982, 114 (01) : 219 - 239
  • [6] Enhanced creation of dispersive monolayer phonons in Xe/Pt(111) by inelastic helium atom scattering at low energies
    Hansen, F. Y.
    Bruch, L. W.
    JOURNAL OF CHEMICAL PHYSICS, 2007, 127 (20):
  • [7] Quasielastic neutron scattering from two-dimensional antiferromagnets at a finite temperature
    Katanin, A.
    Sushkov, O. P.
    PHYSICAL REVIEW B, 2011, 83 (09):
  • [8] Adsorption of Helium Atoms on Two-Dimensional Substrates
    Burganova, Regina
    Lysogorskiy, Yury
    Nedopekin, Oleg
    Tayurskii, Dmitrii
    JOURNAL OF LOW TEMPERATURE PHYSICS, 2016, 185 (5-6) : 392 - 398
  • [9] Adsorption of Helium Atoms on Two-Dimensional Substrates
    Regina Burganova
    Yury Lysogorskiy
    Oleg Nedopekin
    Dmitrii Tayurskii
    Journal of Low Temperature Physics, 2016, 185 : 392 - 398
  • [10] Quasielastic neutron scattering of two-dimensional water in a vermiculite clay
    Swenson, J
    Bergman, R
    Howells, WS
    JOURNAL OF CHEMICAL PHYSICS, 2000, 113 (07): : 2873 - 2879