Construction of Conjugated Carbon Nitride Nanoarchitectures in Solution at Low Temperatures for Photoredox Catalysis

被引：582

作者：

Cui, Yanjuan ^{[1
,2
]}

Ding, Zhengxin ^{[1
,2
]}

Fu, Xianzhi ^{[1
,2
]}

Wang, Xinchen ^{[1
,2
]}

机构：

[1] Fuzhou Univ, Res Inst Photocatalysis, Fujian Prov Key Lab Photocatalysis, State Key Lab Breeding Base, Fuzhou 350002, Peoples R China

[2] Fuzhou Univ, Coll Chem & Chem Engn, Fuzhou 350002, Peoples R China

来源：

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION | 2012年 / 51卷 / 47期

基金：

中国国家自然科学基金;

关键词：

carbon nitride; nanostructures; photocatalysis; solution processing; water splitting; SOLID-STATE NMR; IONOTHERMAL SYNTHESIS; HYDROGEN EVOLUTION; GRAPHITIC FORM; ROUTE; SEMICONDUCTORS; C3N4; CRYSTALLINE;

D O I：

10.1002/anie.201206534

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Hot: Conjugated carbon nitride polymers (LCNs) are synthesized by hot-fluid annealing in one pot. The LCNs possess a narrow band gap, have a complex nanostructure, and show enhanced photochemical performances. The described synthesis approach will allow the rational creation of a wide variety of polymeric carbon nitride semiconductors at low temperature in solutions, with control of structural complexity, electronic structure, and surface functionality. Copyright © 2012 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

引用

页码：11814 / 11818

页数：5

共 49 条

[1] On a new model of the graphitic form of C3N4 [J].

Alves, I ;

Demazeau, G ;

Tanguy, B ;

Weill, F .

SOLID STATE COMMUNICATIONS, 1999, 109 (11) :697-701

[2]

[Anonymous], 2012, Angew. Chem, DOI DOI 10.1002/ange.201106656

[3] Supercritical fluids in heterogeneous catalysis [J].

Baiker, A .

CHEMICAL REVIEWS, 1999, 99 (02) :453-473

[4] Ionothermal Synthesis of Crystalline, Condensed, Graphitic Carbon Nitride [J].

Bojdys, Michael J. ;

Mueller, Jens-Oliver ;

Antonietti, Markus ;

Thomas, Arne .

CHEMISTRY-A EUROPEAN JOURNAL, 2008, 14 (27) :8177-8182

[5] Ordered Mesoporous SBA-15 Type Graphitic Carbon Nitride: A Semiconductor Host Structure for Photocatalytic Hydrogen Evolution with Visible Light [J].

Chen, Xiufang ;

Jun, Young-Si ;

Takanabe, Kazuhiro ;

Maeda, Kazuhiko ;

Domen, Kazunari ;

Fu, Xianzhi ;

Antonietti, Markus ;

Wang, Xinchen .

CHEMISTRY OF MATERIALS, 2009, 21 (18) :4093-4095

[6] Metal-free photocatalytic degradation of 4-chlorophenol in water by mesoporous carbon nitride semiconductors [J].

Cui, Yanjuan ;

Huang, Jianhui ;

Fu, Xianzhi ;

Wang, Xinchen .

CATALYSIS SCIENCE & TECHNOLOGY, 2012, 2 (07) :1396-1402

[7] Solid state NMR of a molecular self-assembly: Multinuclear approach to the cyanuric acid-melamine system [J].

Damodaran, K ;

Sanjayan, GJ ;

Rajamohanan, PR ;

Ganapathy, S ;

Ganesh, KN .

ORGANIC LETTERS, 2001, 3 (12) :1921-1924

[8] Solvothermal processes: a route to the stabilization of new materials [J].

Demazeau, G .

JOURNAL OF MATERIALS CHEMISTRY, 1999, 9 (01) :15-18

[9] A solvothermal synthetic route to prepare polycrystalline carbon nitride [J].

Fu, QA ;

Cao, CB ;

Zhu, HS .

CHEMICAL PHYSICS LETTERS, 1999, 314 (3-4) :223-226

[10] Synthesis of carbon nitrides with graphite-like or onion-like lamellar structures via a solvent-free route at low temperatures [J].

Guo, QX ;

Yang, Q ;

Yi, CQ ;

Zhu, L ;

Xie, Y .

CARBON, 2005, 43 (07) :1386-1391

← 1 2 3 4 5 →