Selective nitrogen doping in graphene for oxygen reduction reactions

被引：172

作者：

Yasuda, Satoshi ^{[1
,2
]}

Yu, Li ^{[1
]}

Kim, Jeheon ^{[1
]}

Murakoshi, Kei ^{[1
]}

机构：

[1] Hokkaido Univ, Fac Sci, Dept Chem, Sapporo, Hokkaido 0600810, Japan

[2] Japan Sci & Technol Agcy, Kawaguchi, Saitama 3320012, Japan

来源：

CHEMICAL COMMUNICATIONS | 2013年 / 49卷 / 83期

关键词：

DOPED GRAPHENE; ACTIVE-SITES; CATALYSTS; OXIDE;

D O I：

10.1039/c3cc45641b

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Nitrogen-doped graphene materials with abundant pyridinic and quaternary nitrogen species were selectively synthesized by thermal surface polymerization of nitrogen-containing aromatic molecules. Catalytic studies revealed that the oxygen reduction by nitrogen-doped graphene, containing pyridinic and quaternary nitrogen species, proceeds via a four- and two-electron reduction pathway, respectively, in alkali-based solutions.

引用

页码：9627 / 9629

页数：3

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