We calculate optical forces and torques exerted on a chiral dipole by chiral light fields and reveal genuine chiral forces in combining the chiral contents of both light field and dipolar matter. Here, the optical chirality is characterized in a general way through the definition of optical chirality density and chirality flow. We show, in particular, that both terms have mechanical effects associated, respectively, with reactive and dissipative components of the chiral forces. Remarkably, these chiral force components are directly related to standard observables: optical rotation for the reactive component and circular dichroism for the dissipative one. As a consequence, the resulting forces and torques are dependent on the enantiomeric form of the chiral dipole. This suggests promising strategies for using chiral light forces to mechanically separate chiral objects according to their enantiomeric form.
机构:
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USAHebrew Univ Jerusalem, Chaim Weizmann Inst Chem, Fritz Haber Ctr Mol Dynam, IL-91904 Jerusalem, Israel
Jain, Prashant K.
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Ghosh, Debraj
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Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USAHebrew Univ Jerusalem, Chaim Weizmann Inst Chem, Fritz Haber Ctr Mol Dynam, IL-91904 Jerusalem, Israel
Ghosh, Debraj
;
Baer, Roi
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Hebrew Univ Jerusalem, Chaim Weizmann Inst Chem, Fritz Haber Ctr Mol Dynam, IL-91904 Jerusalem, IsraelHebrew Univ Jerusalem, Chaim Weizmann Inst Chem, Fritz Haber Ctr Mol Dynam, IL-91904 Jerusalem, Israel
Baer, Roi
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Rabani, Eran
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Tel Aviv Univ, Sackler Fac Sci, Sch Chem, IL-69978 Tel Aviv, IsraelHebrew Univ Jerusalem, Chaim Weizmann Inst Chem, Fritz Haber Ctr Mol Dynam, IL-91904 Jerusalem, Israel
Rabani, Eran
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Alivisatos, A. Paul
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Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USAHebrew Univ Jerusalem, Chaim Weizmann Inst Chem, Fritz Haber Ctr Mol Dynam, IL-91904 Jerusalem, Israel
机构:
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USAHebrew Univ Jerusalem, Chaim Weizmann Inst Chem, Fritz Haber Ctr Mol Dynam, IL-91904 Jerusalem, Israel
Jain, Prashant K.
;
Ghosh, Debraj
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h-index: 0
机构:
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USAHebrew Univ Jerusalem, Chaim Weizmann Inst Chem, Fritz Haber Ctr Mol Dynam, IL-91904 Jerusalem, Israel
Ghosh, Debraj
;
Baer, Roi
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h-index: 0
机构:
Hebrew Univ Jerusalem, Chaim Weizmann Inst Chem, Fritz Haber Ctr Mol Dynam, IL-91904 Jerusalem, IsraelHebrew Univ Jerusalem, Chaim Weizmann Inst Chem, Fritz Haber Ctr Mol Dynam, IL-91904 Jerusalem, Israel
Baer, Roi
;
Rabani, Eran
论文数: 0引用数: 0
h-index: 0
机构:
Tel Aviv Univ, Sackler Fac Sci, Sch Chem, IL-69978 Tel Aviv, IsraelHebrew Univ Jerusalem, Chaim Weizmann Inst Chem, Fritz Haber Ctr Mol Dynam, IL-91904 Jerusalem, Israel
Rabani, Eran
;
Alivisatos, A. Paul
论文数: 0引用数: 0
h-index: 0
机构:
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USAHebrew Univ Jerusalem, Chaim Weizmann Inst Chem, Fritz Haber Ctr Mol Dynam, IL-91904 Jerusalem, Israel