Comparison of Density-Matrix Corrections to Density Functional Theory

被引:14
|
作者
Gibney, Daniel [1 ,2 ]
Boyn, Jan-Niklas [1 ,2 ]
Mazziotti, David A. [1 ,2 ]
机构
[1] Univ Chicago, Dept Chem, Chicago, IL 60637 USA
[2] Univ Chicago, James Franck Inst, Chicago, IL 60637 USA
基金
美国国家科学基金会;
关键词
SELF-INTERACTION ERROR; CONFIGURATION-INTERACTION; ENERGY; THERMOCHEMISTRY; STATES;
D O I
10.1021/acs.jctc.2c00625
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Density functional theory (DFT), one of the most widely utilized methods available to computational chemistry, fails to describe systems with statically correlated electrons. To address this shortcoming, in previous work, we transformed DFT into a one-electron reduced density matrix theory (1-RDMFT) via the inclusion of a quadratic one-electron reduced density matrix (1-RDM) correction. Here, we combine our 1-RDMFT approach with different DFT functionals as well as Hartree-Fock to elucidate the method's dependence on the underlying functional selection. Furthermore, we generalize the information density matrix functional theory (iDMFT), recently developed as a correction to the Hartree-Fock method, by incorporating density functionals in place of the Hartree-Fock functional. We relate iDMFT mathematically to our approach and benchmark the two with a common set of functionals and systems.
引用
收藏
页码:6600 / 6607
页数:8
相关论文
共 50 条
  • [1] Density-matrix functional theory
    Nagy, A
    PHYSICAL REVIEW A, 2002, 66 (02): : 5
  • [2] Comparisons of density-matrix functional theory with density functional theory
    Levy, Mel
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2011, 242
  • [3] Density-matrix functional theory
    Nagy, A.
    2002, American Physical Society (66):
  • [4] Comparison of density-matrix theory and pairing theory
    Tohyama, M
    PROGRESS OF THEORETICAL PHYSICS, 2005, 114 (05): : 1021 - 1034
  • [5] DENSITY-MATRIX AND DENSITY FUNCTIONAL THEORY WITH A GAUSSIAN WAVEPACKET BASIS
    HARRIMAN, JE
    INTERNATIONAL JOURNAL OF QUANTUM CHEMISTRY, 1983, : 501 - 515
  • [6] Correlation energy functional in the density-matrix functional theory
    Yasud, K.
    Physical Review A. Atomic, Molecular, and Optical Physics, 2001, 63 (03): : 325171 - 325171
  • [7] Correlation energy functional in the density-matrix functional theory
    Yasuda, K
    PHYSICAL REVIEW A, 2001, 63 (03): : 1 - 11
  • [8] Benchmark calculations for reduced density-matrix functional theory
    Lathiotakis, N. N.
    Marques, Miguel A. L.
    JOURNAL OF CHEMICAL PHYSICS, 2008, 128 (18):
  • [9] Reduced density-matrix functional theory: Correlation and spectroscopy
    Di Sabatino, S.
    Berger, J. A.
    Reining, L.
    Romaniello, P.
    JOURNAL OF CHEMICAL PHYSICS, 2015, 143 (02):
  • [10] Fractional spin in reduced density-matrix functional theory
    Helbig, N.
    Theodorakopoulos, G.
    Lathiotakis, N. N.
    JOURNAL OF CHEMICAL PHYSICS, 2011, 135 (05):