Nanocrystal photovoltaics: a review of recent progress

被引:72
作者
Stolle, C. Jackson [1 ]
Harvey, Taylor B. [1 ]
Korgel, Brian A. [1 ]
机构
[1] Univ Texas Austin, Texas Mat Inst, Dept Chem Engn, Ctr Nano & Mol Sci & Technol, Austin, TX 78712 USA
基金
美国国家科学基金会;
关键词
QUANTUM-DOT PHOTOVOLTAICS; SOLAR-CELLS; COLLOIDAL NANOCRYSTALS; CUINSE2; NANOCRYSTAL; EFFICIENCY; INKS; PERFORMANCE; DEVICES;
D O I
10.1016/j.coche.2013.03.001
中图分类号
Q81 [生物工程学(生物技术)]; Q93 [微生物学];
学科分类号
071005 ; 0836 ; 090102 ; 100705 ;
摘要
Crystalline inorganic light-absorbing photovoltaic (PV) device layers can be deposited from solution using semiconductor nanocrystal inks to alleviate the problems due to high-temperature and vacuum processing. Inks can be formulated using various semiconductor nanocrystals, so that it is possible to tune band gap energy and target specific compositions of the absorber layers. Nanocrystal PV devices have exhibited efficiencies of up to 7%, and higher efficiencies of 12% have been achieved by sintering the nanocrystals. Recently, nanocrystal quantum dot PV devices have exhibited external quantum efficiencies (EQEs) above 100% due to multiple exciton generation (MEG) and extraction.
引用
收藏
页码:160 / 167
页数:8
相关论文
共 56 条
[1]   Influence of Composition on the Performance of Sintered Cu(In,Ga)Se2 Nanocrystal Thin-Film Photovoltaic Devices [J].
Akhavan, Vahid A. ;
Harvey, Taylor B. ;
Stolle, C. Jackson ;
Ostrowski, David P. ;
Glaz, Micah S. ;
Goodfellow, Brian W. ;
Panthani, Matthew G. ;
Reid, Dariya K. ;
Vanden Bout, David A. ;
Korgel, Brian A. .
CHEMSUSCHEM, 2013, 6 (03) :481-486
[2]   Spray-deposited CuInSe2 nanocrystal photovoltaics [J].
Akhavan, Vahid A. ;
Goodfellow, Brian W. ;
Panthani, Matthew G. ;
Reid, Dariya K. ;
Hellebusch, Danny J. ;
Adachi, Takuji ;
Korgel, Brian A. .
ENERGY & ENVIRONMENTAL SCIENCE, 2010, 3 (10) :1600-1606
[3]   Thickness-limited performance of CuInSe2 nanocrystal photovoltaic devices [J].
Akhavan, Vahid A. ;
Panthani, Matthew G. ;
Goodfellow, Brian W. ;
Reid, Dariya K. ;
Korgel, Brian A. .
OPTICS EXPRESS, 2010, 18 (19) :A411-A420
[4]  
[Anonymous], 2012, SUNSHOT VISION STUDY, DOI DOI 10.2172/1039075
[5]   Comparing Multiple Exciton Generation in Quantum Dots To Impact Ionization in Bulk Semiconductors: Implications for Enhancement of Solar Energy Conversion [J].
Beard, Matthew C. ;
Midgett, Aaron G. ;
Hanna, Mark C. ;
Luther, Joseph M. ;
Hughes, Barbara K. ;
Nozik, Arthur J. .
NANO LETTERS, 2010, 10 (08) :3019-3027
[6]   High-Efficiency Solution-Processed Cu2ZnSn(S,Se)4 Thin-Film Solar Cells Prepared from Binary and Ternary Nanoparticles [J].
Cao, Yanyan ;
Denny, Michael S., Jr. ;
Caspar, Jonathan V. ;
Farneth, William E. ;
Guo, Qijie ;
Ionkin, Alex S. ;
Johnson, Lynda K. ;
Lu, Meijun ;
Malajovich, Irina ;
Radu, Daniela ;
Rosenfeld, H. David ;
Choudhury, Kaushik Roy ;
Wu, Wei .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2012, 134 (38) :15644-15647
[7]   Solution-Processed Nanocrystal Quantum Dot Tandem Solar Cells [J].
Choi, Joshua J. ;
Wenger, Whitney N. ;
Hoffman, Rachel S. ;
Lim, Yee-Fun ;
Luria, Justin ;
Jasieniak, Jacek ;
Marohn, John A. ;
Hanrath, Tobias .
ADVANCED MATERIALS, 2011, 23 (28) :3144-+
[8]   PbSe Nanocrystal Excitonic Solar Cells [J].
Choi, Joshua J. ;
Lim, Yee-Fun ;
Santiago-Berrios, Mitk'El B. ;
Oh, Matthew ;
Hyun, Byung-Ryool ;
Sung, Liangfeng ;
Bartnik, Adam C. ;
Goedhart, Augusta ;
Malliaras, George G. ;
Abruna, Hector D. ;
Wise, Frank W. ;
Hanrath, Tobias .
NANO LETTERS, 2009, 9 (11) :3749-3755
[9]  
Chung C-H, 2012, ADV MAT
[10]   Highly efficient multiple exciton generation in colloidal PbSe and PbS quantum dots [J].
Ellingson, RJ ;
Beard, MC ;
Johnson, JC ;
Yu, PR ;
Micic, OI ;
Nozik, AJ ;
Shabaev, A ;
Efros, AL .
NANO LETTERS, 2005, 5 (05) :865-871