Antibonding Ground States in InAs Quantum-Dot Molecules

被引:100
作者
Doty, M. F. [1 ]
Climente, J. I. [2 ]
Korkusinski, M. [3 ]
Scheibner, M. [1 ]
Bracker, A. S. [1 ]
Hawrylak, P. [3 ]
Gammon, D. [1 ]
机构
[1] USN, Res Lab, Washington, DC 20375 USA
[2] CNR, INFM, Natl Ctr NanoStruct & BioSyst Surfaces, I-41100 Modena, Italy
[3] Natl Res Council Canada, Inst Microstruct Sci, Ottawa, ON K1A 0R6, Canada
关键词
EXCITONS;
D O I
10.1103/PhysRevLett.102.047401
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Coherent tunneling between two InAs quantum dots forms delocalized molecular states. Using magnetophotoluminescence spectroscopy we show that when holes tunnel through a thin barrier, the lowest energy molecular state has bonding orbital character. However, as the thickness of the barrier increases, the molecular ground state changes character from a bonding orbital to an antibonding orbital, confirming recent theoretical predictions. We explain how the spin-orbit interaction causes this counterintuitive reversal by using a four-band k center dot p model and atomistic calculations that account for strain.
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页数:4
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共 17 条
[1]   Spectroscopic study of dark excitons in InxGa1-xAs self-assembled quantum dots by a magnetic-field-induced symmetry breaking [J].
Bayer, M ;
Stern, O ;
Kuther, A ;
Forchel, A .
PHYSICAL REVIEW B, 2000, 61 (11) :7273-7276
[2]   Coupling and entangling of quantum states in quantum dot molecules [J].
Bayer, M ;
Hawrylak, P ;
Hinzer, K ;
Fafard, S ;
Korkusinski, M ;
Wasilewski, ZR ;
Stern, O ;
Forchel, A .
SCIENCE, 2001, 291 (5503) :451-453
[3]   Broken symmetry and quantum entanglement of an exciton in InxGa1-xAs/GaAs quantum dot molecules -: art. no. 075325 [J].
Bester, G ;
Zunger, A ;
Shumway, J .
PHYSICAL REVIEW B, 2005, 71 (07)
[4]   Engineering electron and hole tunneling with asymmetric InAs quantum dot molecules [J].
Bracker, A. S. ;
Scheibner, M. ;
Doty, M. F. ;
Stinaff, E. A. ;
Ponomarev, I. V. ;
Kim, J. C. ;
Whitman, L. J. ;
Reinecke, T. L. ;
Gammon, D. .
APPLIED PHYSICS LETTERS, 2006, 89 (23)
[5]   Theory of valence-band holes as Luttinger spinors in vertically coupled quantum dots [J].
Climente, J. I. ;
Korkusinski, M. ;
Goldoni, G. ;
Hawrylak, P. .
PHYSICAL REVIEW B, 2008, 78 (11)
[6]   Electrically tunable g factors in quantum dot molecular spin states [J].
Doty, M. F. ;
Scheibner, M. ;
Ponomarev, I. V. ;
Stinaff, E. A. ;
Bracker, A. S. ;
Korenev, V. L. ;
Reinecke, T. L. ;
Gammon, D. .
PHYSICAL REVIEW LETTERS, 2006, 97 (19)
[7]   Optical spectra of doubly charged quantum dot molecules in electric and magnetic fields [J].
Doty, M. F. ;
Scheibner, M. ;
Bracker, A. S. ;
Ponomarev, I. V. ;
Reinecke, T. L. ;
Gammon, D. .
PHYSICAL REVIEW B, 2008, 78 (11)
[8]  
*EPAPS, EPRLTAO102044906 EPA
[9]   Strain effects on the electronic structure of strongly coupled self-assembled InAs/GaAs quantum dots:: Tight-binding approach [J].
Jaskolski, W. ;
Zielinski, M. ;
Bryant, Garnett W. ;
Aizpurua, J. .
PHYSICAL REVIEW B, 2006, 74 (19)
[10]   FOURIER-TRANSFORM MAGNETOPHOTOLUMINESCENCE SPECTROSCOPY OF DONOR-BOUND EXCITONS IN GAAS [J].
KARASYUK, VA ;
BECKETT, DGS ;
NISSEN, MK ;
VILLEMAIRE, A ;
STEINER, TW ;
THEWALT, MLW .
PHYSICAL REVIEW B, 1994, 49 (23) :16381-16397