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Gas-liquid interfacial mass transfer in trickle-bed reactors: state-of-the-art correlations
被引:67
|作者:
Iliuta, I
Larachi, F
[1
]
Grandjean, BPA
Wild, G
机构:
[1] Univ Laval, Dept Chem Engn, Quebec City, PQ G1K 7P4, Canada
[2] Univ Laval, CERPIC, Quebec City, PQ G1K 7P4, Canada
[3] ENSIC, CNRS, Lab Sci Genie Chim, F-54001 Nancy, France
基金:
加拿大自然科学与工程研究理事会;
关键词:
trickle-bed reactor;
artificial neural networks;
dimensional analysis;
gas-liquid mass transfer;
correlations;
D O I:
10.1016/S0009-2509(99)00129-3
中图分类号:
TQ [化学工业];
学科分类号:
0817 ;
摘要:
The state-of-the-art of the gas-liquid mass transfer characteristics in trickle-bed reactors was summarized and its quantification methods were reevaluated based on a wide-ranging data base of some 3200 measurements. A set of three unified whole-flow-regime dimensionless correlations for volumetric liquid- and gas-side mass transfer coefficients, and gas-liquid interfacial area, each of which spanned four-order-of-magnitude intervals, were derived. The correlations involved combination of artificial neural networks and dimensional analysis. The dimensionless interfacial area, Sit, and Sit, were expressed as a function of the most pertinent dimensionless groups: Re-L, Re-G, We(L), We(G), Sc-L, Sc-G, St(L), X-G, Mo-L, Fr-L, Eo(M), S-b. (C) 1999 Elsevier Science Ltd. All rights reserved.
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页码:5633 / 5645
页数:13
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