Mesoporous hybrid material composed of Mn3O4 nanoparticles on nitrogen-doped graphene for highly efficient oxygen reduction reaction

被引：237

作者：

Duan, Jingjing ^{[1
]}

Zheng, Yao ^{[1
,2
]}

Chen, Sheng ^{[1
]}

Tang, Youhong ^{[3
,4
]}

Jaroniec, Mietek ^{[5
]}

Qiao, Shizhang ^{[1
]}

机构：

[1] Univ Adelaide, Sch Chem Engn, Adelaide, SA 5005, Australia

[2] Univ Queensland, Australian Inst Bioengn & Nanotechnol, Brisbane, Qld 4072, Australia

[3] Flinders Univ S Australia, Ctr Nano Scale Sci & Technol, Adelaide, SA 5042, Australia

[4] Flinders Univ S Australia, Sch Comp Sci Engn & Math, Adelaide, SA 5042, Australia

[5] Kent State Univ, Dept Chem & Biochem, Kent, OH 44242 USA

来源：

CHEMICAL COMMUNICATIONS | 2013年 / 49卷 / 70期

关键词：

METAL-FREE ELECTROCATALYSTS; FACILE SYNTHESIS; COBALT OXIDE; CARBON; NANOCRYSTALS; CATALYST; SHEETS;

D O I：

10.1039/c3cc43338b

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

The hybrid material composed of Mn3O4 nanoparticles on nitrogen-doped graphene was prepared via a solvothermal process and investigated for the first time as a catalyst for oxygen reduction reaction (ORR). Its high ORR activity, excellent durability and tolerance to methanol make this hybrid material a promising candidate for highly efficient ORR in fuel cells and metal-air batteries.

引用

页码：7705 / 7707

页数：3

共 28 条

[1] Recent Progress in Non-Precious Catalysts for Metal-Air Batteries
Cao, Ruiguo
Lee, Jang-Soo
Liu, Meilin
Cho, Jaephil
[J]. ADVANCED ENERGY MATERIALS, 2012, 2 (07) : 816 - 829
[2] Electrocatalyst approaches and challenges for automotive fuel cells
Debe, Mark K.
[J]. NATURE, 2012, 486 (7401) : 43 - 51
[3] High oxygen-reduction activity and durability of nitrogen-doped graphene
Geng, Dongsheng
Chen, Ying
Chen, Yougui
Li, Yongliang
Li, Ruying
Sun, Xueliang
Ye, Siyu
Knights, Shanna
[J]. ENERGY & ENVIRONMENTAL SCIENCE, 2011, 4 (03) : 760 - 764
[4] Co/CoO Nanoparticles Assembled on Graphene for Electrochemical Reduction of Oxygen
Guo, Shaojun
Zhang, Sen
Wu, Liheng
Sun, Shouheng
[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2012, 51 (47) : 11770 - 11773
[5] Large-Scale Production of Edge-Selectively Functionalized Graphene Nanoplatelets via Ball Milling and Their Use as Metal-Free Electrocatalysts for Oxygen Reduction Reaction
Jeon, In-Yup
Choi, Hyun-Jung
Jung, Sun-Min
Seo, Jeong-Min
Kim, Min-Jung
Dai, Liming
Baek, Jong-Beom
[J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2013, 135 (04) : 1386 - 1393
[6] Gas adsorption characterization of ordered organic-inorganic nanocomposite materials
Kruk, M
Jaroniec, M
[J]. CHEMISTRY OF MATERIALS, 2001, 13 (10) : 3169 - 3183
[7] A Facile and Template-Free Hydrothermal Synthesis of Mn3O4 Nanorods on Graphene Sheets for Supercapacitor Electrodes with Long Cycle Stability
Lee, Jeong Woo
Hall, Anthony S.
Kim, Jong-Duk
Mallouk, Thomas E.
[J]. CHEMISTRY OF MATERIALS, 2012, 24 (06) : 1158 - 1164
[8] Li YG, 2012, NAT NANOTECHNOL, V7, P394, DOI [10.1038/NNANO.2012.72, 10.1038/nnano.2012.72]
[9] Facile Oxygen Reduction on a Three-Dimensionally Ordered Macroporous Graphitic C3N4/Carbon Composite Electrocatalyst
Liang, Ji
Zheng, Yao
Chen, Jun
Liu, Jian
Hulicova-Jurcakova, Denisa
Jaroniec, Mietek
Qiao, Shi Zhang
[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2012, 51 (16) : 3892 - 3896
[10] Strongly Coupled lnorganic/Nanocarbon Hybrid Materials for Advanced Electrocatalysis
Liang, Yongye
Li, Yanguang
Wang, Hailiang
Dai, Hongjie
[J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2013, 135 (06) : 2013 - 2036

← 1 2 3 →