Ultrafast carrier dynamics in thin-films of the topological insulator Bi2Se3

被引:107
作者
Glinka, Yuri D. [1 ,2 ]
Babakiray, Sercan [1 ]
Johnson, Trent A. [1 ]
Bristow, Alan D. [1 ]
Holcomb, Mikel B. [1 ]
Lederman, David [1 ]
机构
[1] W Virginia Univ, Dept Phys & Astron, Morgantown, WV 26506 USA
[2] Natl Acad Sci Ukraine, Inst Phys, UA-03028 Kiev, Ukraine
关键词
DIRAC CONE; EXCITATION;
D O I
10.1063/1.4824821
中图分类号
O59 [应用物理学];
学科分类号
摘要
Transient reflectivity measurements of thin films, ranging from 6 to 40 nm in thickness, of the topological insulator Bi2Se3 reveal a strong dependence of the carrier relaxation time on the film thickness. For thicker films, the relaxation dynamics are similar to those of bulk Bi2Se3, where the contribution of the bulk insulating phase dominates over that of the surface metallic phase. The carrier relaxation time shortens with decreasing film thickness, reaching values comparable to those of noble metals. This effect may result from the hybridization of Dirac cone states at the opposite surfaces for the thinnest films. (C) 2013 AIP Publishing LLC.
引用
收藏
页数:5
相关论文
共 33 条
[1]   Thickness-Independent Transport Channels in Topological Insulator Bi2Se3 Thin Films [J].
Bansal, Namrata ;
Kim, Yong Seung ;
Brahlek, Matthew ;
Edrey, Eliav ;
Oh, Seongshik .
PHYSICAL REVIEW LETTERS, 2012, 109 (11)
[2]   Strong surface scattering in ultrahigh-mobility Bi2Se3 topological insulator crystals [J].
Butch, N. P. ;
Kirshenbaum, K. ;
Syers, P. ;
Sushkov, A. B. ;
Jenkins, G. S. ;
Drew, H. D. ;
Paglione, J. .
PHYSICAL REVIEW B, 2010, 81 (24)
[3]   Experimental Realization of a Three-Dimensional Topological Insulator, Bi2Te3 [J].
Chen, Y. L. ;
Analytis, J. G. ;
Chu, J. -H. ;
Liu, Z. K. ;
Mo, S. -K. ;
Qi, X. L. ;
Zhang, H. J. ;
Lu, D. H. ;
Dai, X. ;
Fang, Z. ;
Zhang, S. C. ;
Fisher, I. R. ;
Hussain, Z. ;
Shen, Z. -X. .
SCIENCE, 2009, 325 (5937) :178-181
[4]   Nonequilibrium electron dynamics in noble metals [J].
Del Fatti, N ;
Voisin, C ;
Achermann, M ;
Tzortzakis, S ;
Christofilos, D ;
Vallée, F .
PHYSICAL REVIEW B, 2000, 61 (24) :16956-16966
[5]   Why gold nanoparticles are more precious than pretty gold: Noble metal surface plasmon resonance and its enhancement of the radiative and nonradiative properties of nanocrystals of different shapes [J].
Eustis, S ;
El-Sayed, MA .
CHEMICAL SOCIETY REVIEWS, 2006, 35 (03) :209-217
[6]   Hot-phonon-assisted absorption at semiconductor heterointerfaces monitored by pump-probe second-harmonic generation [J].
Glinka, Y. D. ;
Tolk, N. H. ;
Liu, X. ;
Sasaki, Y. ;
Furdyna, J. K. .
PHYSICAL REVIEW B, 2008, 77 (11)
[7]   Electro-optic nature of ultrafast pump-probe reflectivity response from multilayer semiconductor heterostructures [J].
Glinka, Y. D. ;
Tolk, N. H. ;
Liu, X. ;
Sasaki, Y. ;
Furdyna, J. K. .
JOURNAL OF APPLIED PHYSICS, 2008, 103 (04)
[8]   Colloquium: Topological insulators [J].
Hasan, M. Z. ;
Kane, C. L. .
REVIEWS OF MODERN PHYSICS, 2010, 82 (04) :3045-3067
[9]   Frequency comb generation at terahertz frequencies by coherent phonon excitation in silicon [J].
Hase, Muneaki ;
Katsuragawa, Masayuki ;
Constantinescu, Anca Monia ;
Petek, Hrvoje .
NATURE PHOTONICS, 2012, 6 (04) :243-247
[10]   Stability of the Bi2Se3(111) topological state: Electron-phonon and electron-defect scattering [J].
Hatch, Richard C. ;
Bianchi, Marco ;
Guan, Dandan ;
Bao, Shining ;
Mi, Jianli ;
Iversen, Bo Brummerstedt ;
Nilsson, Louis ;
Hornekaer, Liv ;
Hofmann, Philip .
PHYSICAL REVIEW B, 2011, 83 (24)