Space-and time-resolved optical investigations on ns-laser produced plasmas on various geological samples

被引:3
作者
Irimiciuc, Stefan [1 ]
Enescu, Florin [2 ,3 ]
Bedelean, Horea [4 ]
Gurlui, Silviu [2 ]
Agop, Maricel [5 ,6 ]
机构
[1] Natl Inst Laser Plasma & Radiat Phys, Laser Dept, Bucharest, Magurele, Romania
[2] Alexandru Ioan Cuza Univ, Fac Phys, LOA SL, Iasi, Romania
[3] Univ Innsbruck, Inst Ion Phys & Appl Phys, 25 Technikerstr, A-6020 Innsbruck, Austria
[4] Babes Bolyai Univ, Dept Geol, Cluj Napoca, Romania
[5] Gh Asachi Tech Univ Iasi, Dept Phys, Iasi 700050, Romania
[6] Romanian Scientists Acad, Bucharest 050094, Romania
关键词
Optical emission spectroscopy; Fast camera imaging; Geological sample; Laser ablation; Melting point; Fractal model; INDUCED BREAKDOWN SPECTROSCOPY; ABLATION; MINERALS; DYNAMICS; LIBS; RAMAN;
D O I
10.1016/j.sab.2020.105904
中图分类号
O433 [光谱学];
学科分类号
0703 ; 070302 ;
摘要
Experimental and theoretical investigations were performed on transient plasmas generated by ns-laser ablation on ten mineral samples. Space-and time-resolved optical emission spectroscopy and ICCD fast camera imaging were implemented to understand the kinetics of the ablated particles and how the samples physical properties can be reflected by those of the plasma plume. Strong correlations were found between the global and individual plasma velocity and the melting temperature of the geomaterials. The thermal energy of the plasma expressed through the excitation temperature of the ejected particle is correlated with the same target physical parameter, results corelated with the presence of strong thermal ejection mechanisms. To better understand the global empirical laws, we implemented the fractal model to interpret the results. The model manages to emulate the target-plasma correlations using a multifractal hydrodynamic approach and adequately calibrating the theoretical model on the empirical tools used to describe the laser produced plasmas.
引用
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页数:10
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