17.6% stabilized efficiency in low-temperature processed planar perovskite solar cells

被引:301
作者
Tao, Chen [1 ]
Neutzner, Stefanie [1 ,2 ]
Colella, Letizia [3 ,4 ]
Marras, Sergio [5 ]
Kandada, Ajay Ram Srimath [1 ]
Gandini, Marina [1 ,2 ]
De Bastiani, Michele [1 ]
Pace, Giuseppina [1 ]
Manna, Liberato [5 ]
Caironi, Mario [1 ]
Bertarelli, Chiara [1 ,3 ]
Petrozza, Annamaria [1 ]
机构
[1] Ctr Nano Sci & Technol PoliMi, Ist Italiano Tecnol, I-20133 Milan, Italy
[2] Politecn Milan, Dipartimento Fis, I-20133 Milan, Italy
[3] Politecn Milan, Dipartimento Chim Mat & Ing Chim G Natta, I-20133 Milan, Italy
[4] INAF, Osservatorio Astron Brera, I-23807 Merate, Italy
[5] Ist Italiano Tecnol, Dept Nanochem, I-16163 Genoa, Italy
关键词
ANOMALOUS HYSTERESIS; INTERFACE; LENGTHS;
D O I
10.1039/c5ee01720c
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
We present here a planar perovskite solar cell with a stabilized power conversion efficiency (PCE) of 17.6% at the maximum power point and a PCE of 17% extracted from quasi-static J-V with an open-circuit voltage of 1.11 V. Such excellent figures of merit can be achieved by engineering a solution-processed electron buffer layer that does not require high temperature steps. A compact thin film of perovskite absorber is grown onto a PCBM-based electron extraction layer by implementing a novel two-step procedure which preserves the soluble organic interlayer during the deposition of successive layers. We demonstrate that efficient charge extraction is the key for high steady state efficiency in perovskite solar cells with a highly integrable architecture.
引用
收藏
页码:2365 / 2370
页数:6
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