Temporal trends in the levels of metals, PCDD/Fs and PCBs in the vicinity of a municipal solid waste incinerator. Preliminary assessment of human health risks

被引:50
作者
Rovira, Joaquim [1 ,2 ]
Vilavert, Lolita [1 ]
Nadal, Marti [1 ]
Schuhmacher, Marta [1 ,2 ]
Domingo, Jose L. [1 ]
机构
[1] Univ Rovira & Virgili, Lab Toxicol & Environm Hlth, Sch Med, IISPV, Reus 43201, Catalonia, Spain
[2] Univ Rovira & Virgili, Environm Engn Lab, Dept Engn Quim, E-43007 Tarragona, Catalonia, Spain
关键词
PCDD/Fs; PCBs; Metals; Human health risks; Municipal solid waste incinerator; DIBENZO-P-DIOXINS; PERSISTENT ORGANIC POLLUTANTS; AMBIENT AIR; POLYCHLORINATED-BIPHENYLS; ATMOSPHERIC DEPOSITION; SPATIAL-DISTRIBUTION; INDUSTRIALIZED CITY; DIETARY EXPOSURE; SOUTH CHINA; SOIL;
D O I
10.1016/j.wasman.2015.05.039
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The concentrations of PCDD/Fs, PCBs, and metals were determined in soil and air samples collected near a municipal solid waste incinerator (MSWI) located in Mataro (Catalonia, Spain), being the health risks for the population living in the vicinity of the facility subsequently assessed. We also established the temporal trends with respect to previous surveys performed in the same zone. In general terms, the highest environmental levels of the pollutants were found in the city of Mataro and were independent on the distance to the MSWI. Soil levels of metals did not show temporal variations between the current and previous campaigns. However, the concentrations of metals in air samples collected in 2011 and 2013, were lower than those found in our 2008 survey. Regarding PCDD/Fs and PCBs, no differences were noted between the levels of the current survey and those corresponding to 2008. Anyhow, the concentrations of metals, PCDD/Fs, and PCBs in soils and air did not exceed the reference values established by regulatory organizations, being also in the low range of other similar studies recently reported. Finally, the human non-carcinogenic and carcinogenic risks due to exposure to metals, PCDD/Fs, and PCBs, were, for the population living in the neighborhood of the MSWI, considered as acceptable according to international standards. (C) 2015 Elsevier Ltd. All rights reserved.
引用
收藏
页码:168 / 175
页数:8
相关论文
共 55 条
[1]  
[Anonymous], 1998, TOX REV HEX CHROM
[2]  
[Anonymous], EPA540R96018
[3]  
[Anonymous], 2009, Risk Assessment Guidance for Superfund
[4]  
[Anonymous], 2008, Document 32008L0050, DOI DOI 10.2766/14352
[5]  
ARC (Agencia de Residus de Catalunya), 2009, VAL GRL MET MET PROT
[6]   Emissions of Polychlorinated Biphenyls, Polychlorinated Dibenzo-p-dioxins, and Polychlorinated Dibenzofurans during 2010 and 2011 in Zurich, Switzerland [J].
Bogdal, Christian ;
Mueller, Claudia E. ;
Buser, Andreas M. ;
Wang, Zhanyun ;
Scheringer, Martin ;
Gerecke, Andreas C. ;
Schmid, Peter ;
Zennegg, Markus ;
MacLeod, Matthew ;
Hungerbuehler, Konrad .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2014, 48 (01) :482-490
[7]   UK concentrations of chromium and chromium (VI), measured as water soluble chromium, in PM10 [J].
Brown, Richard J. C. ;
Van Aswegen, Sivan ;
Webb, William R. ;
Goddard, Sharon L. .
ATMOSPHERIC ENVIRONMENT, 2014, 99 :385-391
[8]   Trends of PCDD/F and PCB concentrations and depositions in ambient air in Northwestern Germany [J].
Bruckmann, Peter ;
Hiester, Ernst ;
Klees, Marcel ;
Zetzsch, Cornelius .
CHEMOSPHERE, 2013, 93 (08) :1471-1478
[9]   Blood levels of polychlorinated dibenzodioxins, polychlorinated dibenzofurans and polychlorinated biphenyls in the general population of a Spanish Mediterranean city. [J].
Ca, CG ;
Kogevinas, M ;
Huici, A ;
Gadea, E ;
Ladona, M ;
Bosch, A ;
Bleda, M .
CHEMOSPHERE, 1998, 36 (03) :419-426
[10]   Point source identification using a simple permutation test: a case study of elevated PCDD/F levels in ambient air and soil and their relation to the distance to a local municipal solid waste incinerator [J].
Chen, Chu-Chih ;
Wu, Kuen-Yuh ;
Chang-Chien, Guo-Ping .
STOCHASTIC ENVIRONMENTAL RESEARCH AND RISK ASSESSMENT, 2011, 25 (07) :929-937