Q Spectroscopy With Superconducting Sensor Microcalorimeters

被引:16
作者
Koehler, K. E. [1 ]
Bennett, D. A. [2 ]
Bond, E. M. [1 ]
Croce, M. P. [1 ]
Dry, D. E. [1 ]
Horansky, R. D. [2 ]
Kotsubo, V. [2 ]
Moody, W. A. [1 ]
Rabin, M. W. [1 ]
Schmidt, D. R. [2 ]
Ullom, J. N. [2 ]
Vale, L. R. [2 ]
机构
[1] Los Alamos Natl Lab, Los Alamos, NM 87545 USA
[2] NIST, Boulder, CO 80305 USA
关键词
Bolometers; cryogenics; radiation detectors; spectroscopy; superconducting devices; ALPHA; RESOLUTION; DETECTORS;
D O I
10.1109/TNS.2012.2225639
中图分类号
TM [电工技术]; TN [电子技术、通信技术];
学科分类号
0808 ; 0809 ;
摘要
The total reaction energy (Q) of individual nuclear decays was measured using microcalorimeters with transition-edge-sensor (TES) thermometers. For alpha-decaying actinides (e.g., U-235, Pu-239, Np-237, Am-241), Q is in the 4-6 MeV range. Nearly all of this energy goes into the relatively light alpha particle, and approximately 100 keV is left over for the much heavier, recoiling daughter atom. Alpha-particle energy spectroscopy with TES-microcalorimeters has shown the ability to simultaneously resolve peaks that overlap in conventional alpha spectroscopy, with resolution now less than 1 keV full-width-at-half-maximum (FWHM) at 5.3 MeV. For total reaction energy spectroscopy, we use the same TES design as our alpha detectors, but embed a small radioactive sample (of about 1 Bq) directly inside an absorber designed to capture all the emitted particles (alpha, recoil nucleus, electrons, X-rays) with near 100% efficiency. We have measured Q-spectra of alpha-decaying isotopes with spectral resolution of 2-3 keV FWHM. For some actinide analytical problems, the Q-spectrum is simpler than the alpha-spectrum: fewer peaks, further apart, and easier to quantify. We will discuss sensor design, methods for embedding radionuclides, and spectral data.
引用
收藏
页码:624 / 629
页数:6
相关论文
共 14 条
[1]  
[Anonymous], 2009, IAEAAQ11
[2]  
BORTELS G, 1987, APPL RADIAT ISOTOPES, V38, P831, DOI 10.1016/0883-2889(87)90180-8
[3]   Defect production efficiency in metals under neutron irradiation [J].
Broeders, CHM ;
Konobeyev, AY .
JOURNAL OF NUCLEAR MATERIALS, 2004, 328 (2-3) :197-214
[4]  
Croce M. P., IEEE T NUCL IN PRESS
[5]  
Edwards K. W., 1965, GEOLOGICAL SURVEY RE
[6]   Measurement of ion cascade energies through resolution degradation of alpha particle microcalorimeters [J].
Horansky, Robert D. ;
Stiehl, Gregory M. ;
Beall, James A. ;
Irwin, Kent D. ;
Plionis, Alexander A. ;
Rabin, Michael W. ;
Ullom, Joel N. .
JOURNAL OF APPLIED PHYSICS, 2010, 107 (04)
[7]   Development of Decay Energy Spectroscopy for Radionuclide Analysis Using Cryogenic 4π Measurements [J].
Jang, Y. S. ;
Lee, S. J. ;
Kim, G. B. ;
Kim, I. H. ;
Kim, M. S. ;
Lee, H. J. ;
Lee, J. S. ;
Lee, K. B. ;
Lee, M. K. ;
Ri, H. C. ;
Yoon, W. S. ;
Kim, Y. H. .
JOURNAL OF LOW TEMPERATURE PHYSICS, 2012, 167 (5-6) :967-972
[8]   Determination of plutonium-240/239 ratios in low activity samples using high resolution alpha-spectrometry [J].
LaMont, SP ;
Glover, SE ;
Filby, RH .
JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY, 1998, 234 (1-2) :195-199
[9]   Cryogenic measurement of alpha decay in a 4π absorber [J].
Lee, Sang-Jun ;
Lee, Min Kyu ;
Jang, Yong Sic ;
Kim, Il Hwan ;
Kim, Sun Kee ;
Lee, June Sur ;
Lee, Kyoung Beom ;
Lee, Young Hwa ;
Kim, Yong-Hamb .
JOURNAL OF PHYSICS G-NUCLEAR AND PARTICLE PHYSICS, 2010, 37 (05)
[10]   Validation study of a new technique for absolute activity measurement with 4π solid angle metallic magnetic calorimeters [J].
Loidl, M. ;
Leblanc, E. ;
Rodrigues, M. ;
Branger, T. ;
Lacour, D. ;
Bouchard, J. ;
Censier, B. .
APPLIED RADIATION AND ISOTOPES, 2008, 66 (6-7) :872-876