Field measurement on the emissions of PM, OC, EC and PAHs from indoor crop straw burning in rural China

被引:92
作者
Wei, Siye [1 ]
Shen, Guofeng [1 ,2 ,3 ]
Zhang, Yanyan [1 ]
Xue, Miao [3 ]
Xie, Han [1 ]
Lin, Pengchuan [1 ]
Chen, Yuanchen [1 ]
Wang, Xilong [1 ]
Tao, Shu [1 ]
机构
[1] Peking Univ, Coll Urban & Environm Sci, Lab Earth Surface Proc, Beijing 100871, Peoples R China
[2] Nanjing Univ, Sch Atmospher Sci, Inst Climate & Global Change Res, Nanjing 210093, Jiangsu, Peoples R China
[3] Jiangsu Acad Environm Sci, Nanjing 210036, Jiangsu, Peoples R China
基金
中国国家自然科学基金; 中国博士后科学基金;
关键词
Indoor crop straw burning; Field measurement; Carbonaceous particulate matter; Polycyclic aromatic hydrocarbons; Influencing factor; POLYCYCLIC AROMATIC-HYDROCARBONS; CARBONACEOUS PARTICULATE MATTER; HOUSEHOLD BIOFUEL COMBUSTION; RESIDENTIAL WOOD COMBUSTION; SIZE DISTRIBUTION; FINE-PARTICLE; MONOXIDE EMISSIONS; AEROSOL EMISSIONS; AIR-POLLUTION; COAL;
D O I
10.1016/j.envpol.2013.07.036
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Field measurements were conducted to measure emission factors of particulate matter (EFPM), organic carbon (EFOC), elemental carbon (EFEC), 28 parent polycyclic aromatic hydrocarbons (EF28pPAHs), and 4 oxygenated PAHs (EF40PAHs) for four types of crop straws burned in two stoves with similar structure but different ages. The average EFPM, EFOC, EFEC, EF28pPAHs, and EF40PAHs were 9.1 +/- 5.7 (1.8-22 as range), 2.6 +/- 2.9 (0.30-12), 1.1 +/- 12 (0.086-5.5), 0.26 +/- 0.19 (0.076-0.96), 0.011 +/- 0.14 (13 x 10(-4) - 0.063) g/kg, respectively. Much high EF28pPAHs was observed in field compared with the laboratory derived EFs and significant difference in EF(28pPAH)s was identified among different crop residues, indicating considerable underestimation when laboratory derived EFs were used in the inventory. The field measured EFPM, EFOC, and EFEC were significantly affected by stove age and the EFs of carbonaceous particles for the 15-year old stove were approximately 2.5 times of those for the 1-year old stove. (C) 2013 Elsevier Ltd. All rights reserved.
引用
收藏
页码:18 / 24
页数:7
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