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A novel cost-effective silica membrane-based process for helium extraction from natural gas
被引:17
作者:
Hamedi, Homa
[1
]
Karimi, Iftekhar A.
[1
]
Gundersen, Truls
[2
]
机构:
[1] Natl Univ Singapore, Dept Chem & Biomol Engn, 4 Engn Dr 4, Singapore 117585, Singapore
[2] Norwegian Univ Sci & Technol NTNU, Dept Energy & Proc Engn, Kolbjorn Hejes V 1A, NO-7491 Trondheim, Norway
关键词:
Helium extraction;
Gas permeation separation;
Sweep gas;
Inorganic membrane;
Organic membrane;
INORGANIC MEMBRANES;
HYDROGEN-PRODUCTION;
RECOVERY;
SEPARATION;
PURIFICATION;
PERFORMANCE;
SIMULATION;
DENSE;
D O I:
10.1016/j.compchemeng.2018.12.013
中图分类号:
TP39 [计算机的应用];
学科分类号:
081203 ;
0835 ;
摘要:
Natural gas reserves with 0.3-2 mol% helium are considered as the only viable source for this noble gas. Currently, cryogenic separation is used to extract helium, but it is energy-intensive. While membrane-based separation is a promising alternative, it is still not considered economical. Even for an inorganic/silica membrane with relatively high selectivity and permeance, a multi-stage membrane system with inter-stage compression is required, which necessitates high CAPEX and OPEX. This study proposes a novel process to enhance the selectivity and permeance of an inorganic/silica membrane system to eliminate the costly inter-stage compression. A 16-24% reduction in the CAPEX and 23-57% in the OPEX are achievable for a natural gas feed with 3-5 mol% helium. In contrast, for a 2 mol% helium feed, the OPEX increases by 34%. However, a 30% decrease in the capital cost outweighs the OPEX increase to make the new process more profitable. (C) 2018 Elsevier Ltd. All rights reserved.
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页码:633 / 638
页数:6
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