Total Synthesis of Aspercyclides A and B via Intramolecular Oxidative Diaryl Ether Formation

被引：25

作者：

Yoshino, Tatsuya ^{[2
]}

Sato, Itaru ^{[1
]}

Hirama, Masahiro ^{[2
]}

机构：

[1] Tohoku Univ, Grad Sch Sci, Dept Chem, Sendai, Miyagi 9808578, Japan

[2] Tohoku Univ, Grad Sch Sci, Res & Analyt Ctr Giant Mol, Sendai, Miyagi 9808578, Japan

来源：

ORGANIC LETTERS | 2012年 / 14卷 / 16期

关键词：

SHARPLESS EPOXIDATION; ENANTIOMERS;

D O I：

10.1021/ol3019727

中图分类号：

O62 [有机化学];

学科分类号：

070303 ; 081704 ;

摘要：

A highly efficient total synthesis of the 11-membered cyclic aspercyclides A (1) and B (2) has been achieved by chemo- and regioselective intramolecular oxidative C-O bond formation from differently substituted diphenols.

引用

页码：4290 / 4292

页数：3

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