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Beyond Impedance Spectroscopy of Perovskite Solar Cells: Insights from the Spectral Correlation of the Electrooptical Frequency Techniques
被引:92
作者:

Bou, Agustin
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Univ Jaume 1, Inst Adv Mat INAM, Castellon de La Plana 12006, Spain Univ Jaume 1, Inst Adv Mat INAM, Castellon de La Plana 12006, Spain

Pockett, Adam
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h-index: 0
机构:
Swansea Univ, Coll Engn, Mat Res Ctr, SPECIFIC, Swansea SA1 8EN, W Glam, Wales Univ Jaume 1, Inst Adv Mat INAM, Castellon de La Plana 12006, Spain

Raptis, Dimitrios
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h-index: 0
机构:
Swansea Univ, Coll Engn, Mat Res Ctr, SPECIFIC, Swansea SA1 8EN, W Glam, Wales Univ Jaume 1, Inst Adv Mat INAM, Castellon de La Plana 12006, Spain

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Carnie, Matthew J.
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Swansea Univ, Coll Engn, Mat Res Ctr, SPECIFIC, Swansea SA1 8EN, W Glam, Wales Univ Jaume 1, Inst Adv Mat INAM, Castellon de La Plana 12006, Spain

Bisquert, Juan
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Univ Jaume 1, Inst Adv Mat INAM, Castellon de La Plana 12006, Spain Univ Jaume 1, Inst Adv Mat INAM, Castellon de La Plana 12006, Spain
机构:
[1] Univ Jaume 1, Inst Adv Mat INAM, Castellon de La Plana 12006, Spain
[2] Swansea Univ, Coll Engn, Mat Res Ctr, SPECIFIC, Swansea SA1 8EN, W Glam, Wales
基金:
英国工程与自然科学研究理事会;
关键词:
INDUCTIVE LOOP;
NEGATIVE CAPACITANCE;
HYSTERESIS;
LIGHT;
TRANSPORT;
MODEL;
D O I:
10.1021/acs.jpclett.0c02459
中图分类号:
O64 [物理化学(理论化学)、化学物理学];
学科分类号:
070304 ;
081704 ;
摘要:
Small perturbation techniques have proven to be useful tools for the investigation of perovskite solar cells. A correct interpretation of the spectra given by impedance spectroscopy (IS), intensity-modulated photocurrent spectroscopy (IMPS), and intensity-modulated photovoltage spectroscopy (IMVS) is key for the understanding of device operation. The utilization of a correct equivalent circuit to extract real parameters is essential to make this good interpretation. In this work, we present an equivalent circuit, which is able to reproduce the general and the exotic behaviors found in impedance spectra. From the measurements, we demonstrate that the midfrequency features that may appear to depend on the active layer thickness, and we also prove the spectral correlation of the three techniques that has been suggested theoretically.
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收藏
页码:8654 / 8659
页数:6
相关论文
共 31 条
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