Numerical simulation of flow field and residence time of nanoparticles in a 1000-ton industrial multi-jet combustion reactor

In this work, by establishing a three-dimensional physical model of a 1000-ton industrial multi-jet combustion reactor, a hexahedral structured grid was used to discretize the model. Combined with realizable k-e model, eddy-dissipation-concept, discrete-ordinate radiation model, hydrogen 19-step detailed reaction mechanism, air age user-defined-function, velocity field, temperature field, concentration field and gas arrival time in the reactor were numerically simulated. The Euler-Lagrange method combined with the discrete-phase-model was used to reveal the flow characteristics of particles in the reactor, and based on this, the effects of the reactor aspect ratios, central jet gas velocity and particle size on the flow field characteristics and particle back-mixing degree in the reactor were investigated. The results show that with the decrease of aspect ratio in the combustion reactors, the velocity and temperature attenuation in the reactor are intensified, the vortex phenomenon is aggravated, and the residence time distribution of nanoparticles is more dispersed. With the increase in the central jet gas velocities in reactors, the vortex lengthens along the axis, the turbulence intensity increases, and the residence time of particles decreases. The back-mixing degree and residence time of particles in the reactor also decrease with the increase in particle size. The simulation results can provide reference for the structural regulation of nanoparticles and the structural design of combustion reactor in the process of gas combustion synthesis. (c) 2021 The Chemical Industry and Engineering Society of China, and Chemical Industry Press Co., Ltd. All rights reserved.