Organophosphate and brominated flame retardants in Australian indoor environments: Levels, sources, and preliminary assessment of human exposure

被引:135
|
作者
He, Chang [1 ]
Wang, Xianyu [1 ]
Phong Thai [2 ]
Baduel, Christine [1 ,3 ]
Gallen, Christie [1 ]
Banks, Andrew [1 ]
Bainton, Paul [4 ]
English, Karin [5 ,6 ]
Mueller, Jochen F. [1 ]
机构
[1] Univ Queensland, QAEHS, Brisbane, Qld, Australia
[2] Queensland Univ Technol, Int Lab Air Qual & Hlth, Brisbane, Qld, Australia
[3] Univ Claude Bernard Lyon 1, Univ Lyon, Inst Sci Analyt, CNRS,ENS Lyon,UMR 5280, 5 Rue Doua, F-69100 Villeurbanne, France
[4] Dept Environm & Energy, GPO Box 787, Canberra, ACT 2601, Australia
[5] Univ Queensland, Sch Med, Brisbane, Qld, Australia
[6] Univ Queensland, Child Hlth Res Ctr, Childrens Hlth & Environm Program, Brisbane, Qld, Australia
基金
澳大利亚研究理事会;
关键词
OPFRs; PBDEs; Alternative flame retardants; Indoor dust and air; Plasticizer; POLYBROMINATED DIPHENYL ETHERS; IN-HOUSE DUST; PASSIVE AIR; ORGANIC CONTAMINANTS; GAS-CHROMATOGRAPHY; CONSUMER PRODUCTS; OUTDOOR AIR; PHASE-OUT; PBDES; PLASTICIZERS;
D O I
10.1016/j.envpol.2017.12.017
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Concentrations of nine organophosphate flame retardants (OPFRs) and eight polybrominated diphenyl ethers (PBDEs) were measured in samples of indoor dust (n = 85) and air (n = 45) from Australian houses, offices, hotels, and transportation (buses, trains, and aircraft). All target compounds were detected in indoor dust and air samples. Median Sigma(9)OPFRs concentrations were 40 gig in dust and 44 ng/m(3) in indoor air, while median Sigma 8PBDEs concentrations were 2.1 mu g/g and 0.049 ng/m(3). Concentrations of FRs were higher in rooms that contained carpet, air conditioners, and various electronic items. Estimated daily intakes in adults are 14000 pg/kg body weight/day and 330 pg/kg body weight/day for Sigma(9)OPFRs and Sigma 8PBDEs, respectively. Our results suggest that for the volatile FRs such as tris(2-chloroethyl) phosphate (TCEP) and TCIPP, inhalation is expected to be the more important intake pathway compared to dust ingestion and dermal contact. (C) 2018 Elsevier Ltd. All rights reserved.
引用
收藏
页码:670 / 679
页数:10
相关论文
共 50 条
  • [31] Human health risks from brominated flame retardants and polycyclic aromatic hydrocarbons in indoor dust
    Al-Harbi, Meshari
    Al-Enzi, Eman
    Al-Mutairi, Hessa
    Whalen, Joann K.
    CHEMOSPHERE, 2021, 282
  • [32] Concentrations of organophosphate esters and brominated flame retardants in German indoor dust samples
    Brommer, Sandra
    Harrad, Stuart
    Van den Eede, Nele
    Covaci, Adrian
    JOURNAL OF ENVIRONMENTAL MONITORING, 2012, 14 (09): : 2482 - 2487
  • [33] High levels of flame retardants in vehicle dust indicate ongoing use of brominated and organophosphate flame retardants in vehicle interiors
    Svobodova, Petra
    Jilkova, Simona Rozarka
    Kohoutek, Jiri
    Audy, Ondrej
    Senk, Petr
    Melymuk, Lisa
    ENVIRONMENTAL MONITORING AND ASSESSMENT, 2025, 197 (04)
  • [34] Brominated flame retardants - Exposure and risk assessment for the general population
    Fromme, H.
    Becher, G.
    Hilger, B.
    Voelkel, W.
    INTERNATIONAL JOURNAL OF HYGIENE AND ENVIRONMENTAL HEALTH, 2016, 219 (01) : 1 - 23
  • [35] A review on sources of brominated flame retardants and routes of human exposure with emphasis on polybrominated diphenyl ethers
    Daso, Adegbenro P.
    Fatoki, Olalekan S.
    Odendaal, James P.
    Okonkwo, Jonathan O.
    ENVIRONMENTAL REVIEWS, 2010, 18 : 239 - 254
  • [36] Brominated flame retardants in Belgian home-produced eggs: Levels and contamination sources
    Covaci, Adrian
    Roosens, Laurence
    Dirtu, Alin C.
    Waegeneers, Nadia
    Van Overmeire, Ilse
    Neels, Hugo
    Goeyens, Leo
    SCIENCE OF THE TOTAL ENVIRONMENT, 2009, 407 (15) : 4387 - 4396
  • [37] Exposure assessment and health risk of poly-brominated diphenyl ether (PBDE) flame retardants in the indoor environment of elementary school students in Korea
    Lim, Young-Wook
    Kim, Ho-Hyun
    Lee, Chung-Soo
    Shin, Dong-Chun
    Chang, Yoon-Seok
    Yang, Ji-Yeon
    SCIENCE OF THE TOTAL ENVIRONMENT, 2014, 470 : 1376 - 1389
  • [38] Occurrence and human exposure assessment of organophosphate flame retardants in indoor dust from various microenvironments of the Rhine/Main region, Germany
    Zhou, L.
    Hiltscher, M.
    Puettmann, W.
    INDOOR AIR, 2017, 27 (06) : 1113 - 1127
  • [39] Measurements of Selected Brominated Flame Retardants in Nursing Women: Implications for Human Exposure
    Zhou, Simon Ningsun
    Buchar, Angelina
    Siddique, Shabana
    Takser, Larissa
    Abdelouahab, Nadia
    Zhu, Jiping
    ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2014, 48 (15) : 8873 - 8880
  • [40] Measurements of Parameters Controlling the Emissions of Organophosphate Flame Retardants in Indoor Environments
    Liang, Yirui
    Liu, Xiaoyu
    Allen, Matthew R.
    ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2018, 52 (10) : 5821 - 5829