Mass transfer formulation for polymer electrolyte membrane fuel cell cathode

被引:11
作者
Beale, Steven B. [1 ]
机构
[1] Forschungszentrum Julich, Inst Energy & Climate Res, IEK 3, D-92425 Julich, Germany
关键词
Fuel cells; Transport phenomena; Mass transfer; Concentration polarisation; Diffusion over-potential; MODEL; TRANSPORT; LAYERS;
D O I
10.1016/j.ijhydene.2015.05.074
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
A standard mechanical engineering mass transfer analysis is adapted to obtain performance calculations for the cathode of a typical polymer electrolyte membrane fuel cell. Mathematical details are provided and sample calculations performed, based on a number of simplifying assumptions. The relative advantages of low and high-mass transfer formulations are critically appraised and compared to a highly-simplified method. Copyright (C) 2015, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码:11641 / 11650
页数:10
相关论文
共 24 条
[1]   Conjugate mass transfer in gas channels and diffusion layers of fuel cells [J].
Beale, S. B. .
JOURNAL OF FUEL CELL SCIENCE AND TECHNOLOGY, 2007, 4 (01) :1-10
[2]   TWO-PHASE FLOW AND MASS TRANSFER WITHIN THE DIFFUSION LAYER OF A POLYMER ELECTROLYTE MEMBRANE FUEL CELL [J].
Beale, S. B. ;
Schwarz, D. H. ;
Malin, M. R. ;
Spalding, D. B. .
COMPUTATIONAL THERMAL SCIENCES, 2009, 1 (02) :105-120
[3]   Calculation procedure for mass transfer in fuel cells [J].
Beale, SB .
JOURNAL OF POWER SOURCES, 2004, 128 (02) :185-192
[4]   MATHEMATICAL-MODEL OF A GAS-DIFFUSION ELECTRODE BONDED TO A POLYMER ELECTROLYTE [J].
BERNARDI, DM ;
VERBRUGGE, MW .
AICHE JOURNAL, 1991, 37 (08) :1151-1163
[5]   A 3D, multiphase, multicomponent model of the cathode and anode of a PEM fuel cell [J].
Berning, T ;
Djilali, N .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2003, 150 (12) :A1589-A1598
[6]  
Bird R.B., 2001, Transport Phenomena, Vsecond, DOI DOI 10.1002/AIC.690070245
[7]   A review on water balance in the membrane electrode assembly of proton exchange membrane fuel cells [J].
Dai, Wei ;
Wang, Haijiang ;
Yuan, Xiao-Zi ;
Martin, Jonathan J. ;
Yang, Daijun ;
Qiao, Jinli ;
Ma, Jianxin .
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2009, 34 (23) :9461-9478
[8]   Multimodal mass transfer in solid-oxide fuel-cells [J].
Garcia-Camprubi, M. ;
Sanchez-Insa, A. ;
Fueyo, N. .
CHEMICAL ENGINEERING SCIENCE, 2010, 65 (05) :1668-1677
[9]   A comparison of different approaches to modelling the PEMFC catalyst layer [J].
Harvey, D. ;
Pharoah, J. G. ;
Karan, K. .
JOURNAL OF POWER SOURCES, 2008, 179 (01) :209-219
[10]  
Kays W.M., 2011, Convective heat and mass transfer