Mass transfer formulation for polymer electrolyte membrane fuel cell cathode

被引：11
作者：
Beale, Steven B. [1 ]
机构：
[1] Forschungszentrum Julich, Inst Energy & Climate Res, IEK 3, D-92425 Julich, Germany
来源：
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY | 2015年 / 40卷 / 35期
关键词：
Fuel cells; Transport phenomena; Mass transfer; Concentration polarisation; Diffusion over-potential; MODEL; TRANSPORT; LAYERS;
D O I：
10.1016/j.ijhydene.2015.05.074
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
A standard mechanical engineering mass transfer analysis is adapted to obtain performance calculations for the cathode of a typical polymer electrolyte membrane fuel cell. Mathematical details are provided and sample calculations performed, based on a number of simplifying assumptions. The relative advantages of low and high-mass transfer formulations are critically appraised and compared to a highly-simplified method. Copyright (C) 2015, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码：11641 / 11650
页数：10
相关论文
共 24 条
  • [1] Conjugate mass transfer in gas channels and diffusion layers of fuel cells
    Beale, S. B.
    [J]. JOURNAL OF FUEL CELL SCIENCE AND TECHNOLOGY, 2007, 4 (01): : 1 - 10
  • [2] TWO-PHASE FLOW AND MASS TRANSFER WITHIN THE DIFFUSION LAYER OF A POLYMER ELECTROLYTE MEMBRANE FUEL CELL
    Beale, S. B.
    Schwarz, D. H.
    Malin, M. R.
    Spalding, D. B.
    [J]. COMPUTATIONAL THERMAL SCIENCES, 2009, 1 (02): : 105 - 120
  • [3] Calculation procedure for mass transfer in fuel cells
    Beale, SB
    [J]. JOURNAL OF POWER SOURCES, 2004, 128 (02) : 185 - 192
  • [4] MATHEMATICAL-MODEL OF A GAS-DIFFUSION ELECTRODE BONDED TO A POLYMER ELECTROLYTE
    BERNARDI, DM
    VERBRUGGE, MW
    [J]. AICHE JOURNAL, 1991, 37 (08) : 1151 - 1163
  • [5] A 3D, multiphase, multicomponent model of the cathode and anode of a PEM fuel cell
    Berning, T
    Djilali, N
    [J]. JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2003, 150 (12) : A1589 - A1598
  • [6] Bird R.B., 2001, Transport Phenomena, Vsecond, DOI DOI 10.1002/AIC.690070245
  • [7] A review on water balance in the membrane electrode assembly of proton exchange membrane fuel cells
    Dai, Wei
    Wang, Haijiang
    Yuan, Xiao-Zi
    Martin, Jonathan J.
    Yang, Daijun
    Qiao, Jinli
    Ma, Jianxin
    [J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2009, 34 (23) : 9461 - 9478
  • [8] Multimodal mass transfer in solid-oxide fuel-cells
    Garcia-Camprubi, M.
    Sanchez-Insa, A.
    Fueyo, N.
    [J]. CHEMICAL ENGINEERING SCIENCE, 2010, 65 (05) : 1668 - 1677
  • [9] A comparison of different approaches to modelling the PEMFC catalyst layer
    Harvey, D.
    Pharoah, J. G.
    Karan, K.
    [J]. JOURNAL OF POWER SOURCES, 2008, 179 (01) : 209 - 219
  • [10] Kays W.M., 2011, Convective heat and mass transfer
123