Hierarchically Macro-Mesoporous Pt/γ-Al2O3 Composite Microspheres for Efficient Formaldehyde Oxidation at Room Temperature

被引:131
作者
Nie, Longhui [1 ,3 ]
Meng, Aiyun [1 ]
Yu, Jiaguo [1 ]
Jaroniec, Mietek [2 ]
机构
[1] Wuhan Univ Technol, State Key Lab Adv Technol Mat Synth & Proc, Wuhan 430070, Peoples R China
[2] Kent State Univ, Dept Chem & Biochem, Kent, OH 44242 USA
[3] Hubei Univ Technol, Sch Chem & Chem Engn, Wuhan 430068, Peoples R China
来源
SCIENTIFIC REPORTS | 2013年 / 3卷
关键词
PHOTOCATALYTIC ACTIVITY; CATALYTIC PERFORMANCE; PT/TIO2; CATALYST; HOLLOW SPHERES; FABRICATION; NANOSHEETS; REMOVAL; ALUMINA; SULFUR; AL2O3;
D O I
10.1038/srep03215
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Room temperature catalytic oxidation by noble metals is considered to be the most promising strategy for the removal of HCHO, which is one of the major indoor air pollutants. Hierarchically macro-mesoporous structured Pt/gamma-Al2O3 hollow spheres with open and accessible pores were synthesized and used for catalytic oxidative decomposition of HCHO at room temperature. The prepared composite hollow spheres showed higher catalytic activity than the conventional nanoparticle supports, which is mainly due to their hierarchical macro-mesoporous structure facilitating diffusion of reactants and products, and the high dispersion of accessible catalytic Pt nanoparticles. This work may contribute to the development of hierarchically structured materials and high-performance catalysts for indoor air purification and related catalytic processes.
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页数:6
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