Ag2S quantum dots and N3 dye co-sensitized TiO2 nanotube arrays for a solar cell

被引:31
作者
Ji, Gangqiang [1 ]
Liu, Zhongqing [1 ]
Guan, Debin [2 ,3 ]
Yang, Yuntao [2 ,3 ]
机构
[1] Sichuan Univ, Coll Chem Engn, Chengdu 610065, Sichuan, Peoples R China
[2] China Acad Engn Phys, Inst Chem Mat, Mianyang 621900, Peoples R China
[3] China Acad Engn Phys, Adv Mat Res Ctr, Mianyang 621900, Peoples R China
关键词
TiO2 nanotube arrays; Ag2S quantum dots; S-CBD; Co-sensitized solar cell; Photoelectric conversion; FABRICATION; ELECTRODEPOSITION; PHOTOELECTRODES;
D O I
10.1016/j.apsusc.2013.06.035
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Ag2S quantum dots (QDs) and N3 dye co-sensitized TiO2 nanotube arrays (Ag2S-N3-TNAs) were prepared by the processes of anodization method followed by sequential chemical bath deposition (S-CBD) approach and dye sensitization, using FTO-based titanium film formed by vacuum ion coating method as a precursor. XRD, EDS, FE-SEM, TEM, UV-vis diffuse reflectance and photo electrochemical measurements were used to characterize the samples. Fabricated co-sensitized solar cell prototype exhibited a photocurrent density of 10.2 mA cm(-2) and a power conversion efficiency of 4.40% based solar cells, which is higher than that of N3-sensitized TiO2 nanotube arrays (N3-TNAs) (8.5 mA cm-2 and 3.64%) under AM 1.5 light irradiation. (C) 2013 Elsevier B.V. All rights reserved.
引用
收藏
页码:695 / 699
页数:5
相关论文
共 20 条
[1]   Photovoltaic efficiency on dye-sensitized solar cells (DSSC) assembled using Ga-incorporated TiO2 materials [J].
Chae, Jinho ;
Kim, Dong Young ;
Kim, Sujung ;
Kang, Misook .
JOURNAL OF INDUSTRIAL AND ENGINEERING CHEMISTRY, 2010, 16 (06) :906-911
[2]   Photoelectrode thin film of dye-sensitized solar cell fabricated by anodizing method and spin coating and electrochemical impedance properties of DSSC [J].
Chang, Ho ;
Chen, Chih-Hao ;
Kao, Mu-Jung ;
Chien, Shu-Hua ;
Chou, Cheng-Yi .
APPLIED SURFACE SCIENCE, 2013, 275 :252-257
[3]  
Gouma PI, 2000, J AM CERAM SOC, V83, P1007, DOI 10.1111/j.1151-2916.2000.tb01320.x
[4]   Improved conversion efficiency of dye-sensitized solar cell based on the porous anodic TiO2 nanotubes [J].
He, Weizhen ;
Qiu, Jijun ;
Choi, Su-Kyung ;
Kim, Whi-Dong ;
Lee, Jae-Ho ;
Kim, Yang-Do ;
Kim, Soo-Hyung ;
Kim, Hyung-Kook ;
Hwang, Yoon-Hwae .
CURRENT APPLIED PHYSICS, 2011, 11 (03) :S320-S323
[5]   Electrodeposition preparation of octahedral-Cu2O-loaded TiO2 nanotube arrays for visible light-driven photocatalysis [J].
Huang, L. ;
Zhang, S. ;
Peng, F. ;
Wang, H. ;
Yu, H. ;
Yang, J. ;
Zhang, S. ;
Zhao, H. .
SCRIPTA MATERIALIA, 2010, 63 (02) :159-161
[6]   Nanostructured photovoltaic cell of the type titanium dioxide, cadmium sulfide thin coating, and copper thiocyanate showing high quantum efficiency [J].
Larramona, G ;
Choné, C ;
Jacob, A ;
Sakakura, D ;
Delatouche, B ;
Péré, D ;
Cieren, X ;
Nagino, M ;
Bayón, R .
CHEMISTRY OF MATERIALS, 2006, 18 (06) :1688-1696
[7]   Ordered Crystalline TiO2 Nanotube Arrays on Transparent FTO Glass for Efficient Dye-Sensitized Solar Cells [J].
Lei, Bing-Xin ;
Liao, Jin-Yun ;
Zhang, Ran ;
Wang, Jing ;
Su, Cheng-Yong ;
Kuang, Dai-Bin .
JOURNAL OF PHYSICAL CHEMISTRY C, 2010, 114 (35) :15228-15233
[8]   Fabrication of TiO2 nanotube arrays by electrochemical anodization in an NH4F/H3PO4 electrolyte [J].
Liu, Rui ;
Yang, Wein-Duo ;
Qiang, Liang-Sheng ;
Wu, Jian-Fu .
THIN SOLID FILMS, 2011, 519 (19) :6459-6466
[9]   Theoretical evidence of multiple dye regeneration mechanisms in dye-sensitized solar cells [J].
Liu, Tao ;
Troisi, Alessandro .
CHEMICAL PHYSICS LETTERS, 2013, 570 :159-162
[10]   Facile fabrication of well-dispersed silver nanoparticles loading on TiO2 nanotube arrays by electrodeposition [J].
Liu, Xu ;
Liu, Zhongqing ;
Hao, Shixiong ;
Chu, Wei .
MATERIALS LETTERS, 2012, 80 :66-68