A carbon-based photocatalyst efficiently converts CO2 to CH4 and C2H2 under visible light

被引:62
|
作者
Wu, Tongshun [1 ]
Zou, Luyi [2 ]
Han, Dongxue [1 ]
Li, Fenghua [1 ]
Zhang, Qixian [1 ]
Niu, Li [1 ]
机构
[1] Chinese Acad Sci, Changchun Inst Appl Chem, Engn Lab Modern Analyt Tech, State Key Lab Electroanalyt Chem, Changchun 130022, Peoples R China
[2] Jilin Univ, Inst Theoret Chem, State Key Lab Theoret & Computat Chem, Changchun 130023, Peoples R China
关键词
SOLAR FUEL PRODUCTION; BILAYER GRAPHENE; REDUCTION; DIOXIDE; METHANE; WATER; HYDROCARBONS; CHALLENGE; OXIDATION; CHEMICALS;
D O I
10.1039/c3gc42454e
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Novel photocatalysts consisting of porphyrin and graphene have been designed to reduce CO2 to hydrocarbons under visible light. These catalysts can (i) effectively reduce CO2 to hydrocarbons, particularly to C2H2; and (ii) selectively control the transfer of photo-generated electrons from graphene to CO2 rather than to H2O.
引用
收藏
页码:2142 / 2146
页数:5
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