Three-Dimensional N-Doped Graphene Hydrogel/NiCo Double Hydroxide Electrocatalysts for Highly Efficient Oxygen Evolution

被引:551
作者
Chen, Sheng [1 ]
Duan, Jingjing [1 ]
Jaroniec, Mietek [2 ]
Qiao, Shi Zhang [1 ]
机构
[1] Univ Adelaide, Sch Chem Engn, Adelaide, SA 5005, Australia
[2] Kent State Univ, Dept Chem & Biochem, Kent, OH USA
基金
澳大利亚研究理事会;
关键词
metal oxides; nanostructures; N-doped graphene; oxygen evolution reaction; WATER OXIDATION; ELECTRODES; FOAMS; OXIDE;
D O I
10.1002/anie.201306166
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A highly hydrated structure was fabricated for catalyzing the oxygen evolution reaction (OER), which demonstrated significantly enhanced catalytic activity, favorable kinetics, and strong durability. The enhanced performance is correlated with the dual-active-site mechanism, and high hydrophilicity of the electrode can dramatically expedite the process of water oxidation into molecular oxygen. Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
引用
收藏
页码:13567 / 13570
页数:4
相关论文
共 21 条
  • [1] INNER AND OUTER ACTIVE SURFACE OF RUO2 ELECTRODES
    ARDIZZONE, S
    FREGONARA, G
    TRASATTI, S
    [J]. ELECTROCHIMICA ACTA, 1990, 35 (01) : 263 - 267
  • [2] Building better batteries
    Armand, M.
    Tarascon, J. -M.
    [J]. NATURE, 2008, 451 (7179) : 652 - 657
  • [3] Highly Efficient Electrocatalytic Hydrogen Production by MoSx Grown on Graphene-Protected 3D Ni Foams
    Chang, Yung-Huang
    Lin, Cheng-Te
    Chen, Tzu-Yin
    Hsu, Chang-Lung
    Lee, Yi-Hsien
    Zhang, Wenjing
    Wei, Kung-Hwa
    Li, Lain-Jong
    [J]. ADVANCED MATERIALS, 2013, 25 (05) : 756 - 760
  • [4] Graphene Hydrogels Deposited in Nickel Foams for High-Rate Electrochemical Capacitors
    Chen, Ji
    Sheng, Kaixuan
    Luo, Peihui
    Li, Chun
    Shi, Gaoquan
    [J]. ADVANCED MATERIALS, 2012, 24 (33) : 4569 - 4573
  • [5] Water Oxidation Electrocatalyzed by an Efficient Mn3O4/CoSe2 Nanocomposite
    Gao, Min-Rui
    Xu, Yun-Fei
    Jiang, Jun
    Zheng, Ya-Rong
    Yu, Shu-Hong
    [J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2012, 134 (06) : 2930 - 2933
  • [6] An Advanced Ni-Fe Layered Double Hydroxide Electrocatalyst for Water Oxidation
    Gong, Ming
    Li, Yanguang
    Wang, Hailiang
    Liang, Yongye
    Wu, Justin Z.
    Zhou, Jigang
    Wang, Jian
    Regier, Tom
    Wei, Fei
    Dai, Hongjie
    [J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2013, 135 (23) : 8452 - 8455
  • [7] Powering the planet with solar fuel
    Gray, Harry B.
    [J]. NATURE CHEMISTRY, 2009, 1 (01) : 7 - 7
  • [8] PREPARATION OF GRAPHITIC OXIDE
    HUMMERS, WS
    OFFEMAN, RE
    [J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1958, 80 (06) : 1339 - 1339
  • [9] NixCo3-xO4 Nanowire Arrays for Electrocatalytic Oxygen Evolution
    Li, Yanguang
    Hasin, Panitat
    Wu, Yiying
    [J]. ADVANCED MATERIALS, 2010, 22 (17) : 1926 - +
  • [10] Mirzakulova E, 2012, NAT CHEM, V4, P794, DOI [10.1038/NCHEM.1439, 10.1038/nchem.1439]