Severe haze in northern China: A synergy of anthropogenic emissions and atmospheric processes

被引:699
作者
An, Zhisheng [1 ,2 ,3 ,4 ,5 ]
Huang, Ru-Jin [1 ,2 ,3 ,4 ,5 ]
Zhang, Renyi [6 ,7 ]
Tie, Xuexi [1 ,3 ]
Li, Guohui [1 ,2 ,3 ]
Cao, Junji [1 ,2 ,3 ]
Zhou, Weijian [1 ,2 ,4 ,5 ]
Shi, Zhengguo [1 ,2 ,8 ]
Han, Yongming [1 ,2 ,3 ,8 ]
Gu, Zhaolin [8 ]
Ji, Yuemeng [6 ,9 ]
机构
[1] Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian 710061, Shaanxi, Peoples R China
[2] Chinese Acad Sci, Ctr Excellence Quaternary Sci & Global Change, Xian 710061, Shaanxi, Peoples R China
[3] Chinese Acad Sci, Inst Earth Environm, Key Lab Aerosol Chem & Phys, Xian 710061, Shaanxi, Peoples R China
[4] Beijing Normal Univ, Interdisciplinary Res Ctr Earth Sci Frontier, Beijing 100875, Peoples R China
[5] Pilot Natl Lab Marine Sci & Technol Qingdao, Open Studio Ocean Continental Climate & Environm, Qingdao 266061, Peoples R China
[6] Texas A&M Univ, Dept Atmospher Sci, College Stn, TX 77843 USA
[7] Texas A&M Univ, Dept Chem, College Stn, TX 77843 USA
[8] Xi An Jiao Tong Univ, Dept Earth & Environm Sci, Xian 710049, Shaanxi, Peoples R China
[9] Guangdong Univ Technol, Sch Environm Sci & Engn, Guangzhou Key Lab Environm Catalysis & Pollut Con, Guangzhou 510006, Guangdong, Peoples R China
基金
中国国家自然科学基金;
关键词
severe haze; synergetic effects; anthropogenic emission; atmospheric chemistry; climate change; TIME CHEMICAL-CHARACTERIZATION; AIR-POLLUTANT EMISSIONS; FINE PARTICULATE MATTER; ASIAN SUMMER MONSOON; PARTICLE FORMATION; REGIONAL TRANSPORT; BOUNDARY-LAYER; BLACK CARBON; HEAVY HAZE; AEROSOL COMPOSITION;
D O I
10.1073/pnas.1900125116
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Regional severe haze represents an enormous environmental problem in China, influencing air quality, human health, ecosystem, weather, and climate. These extremes are characterized by exceedingly high concentrations of fine particulate matter (smaller than 2.5 mu m, or PM2.5) and occur with extensive temporal (on a daily, weekly, to monthly timescale) and spatial (over a million square kilometers) coverage. Although significant advances have been made in field measurements, model simulations, and laboratory experiments for fine PM over recent years, the causes for severe haze formation have not yet to be systematically/comprehensively evaluated. This review provides a synthetic synopsis of recent advances in understanding the fundamental mechanisms of severe haze formation in northern China, focusing on emission sources, chemical formation and transformation, and meteorological and climatic conditions. In particular, we highlight the synergetic effects from the interactions between anthropogenic emissions and atmospheric processes. Current challenges and future research directions to improve the understanding of severe haze pollution as well as plausible regulatory implications on a scientific basis are also discussed.
引用
收藏
页码:8657 / 8666
页数:10
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